The invention discloses a method for electroplating a Ni-Cr-PTFE composite coating in ionic liquid. In a non-water system and an inert-gas atmosphere, [BMIM]NiCl3 liquid containing nickel ions, [BMIM]CrCl4 liquid containing chromium ions, LiCl, PTFE and N,N-dimethyldodecylamine oxide (OB-2) are added into a certain amount of mixed solvent of 1-ethyl-3-methylimidazolium chlorine (EMIMCI) and ethylene glycol (EG), mechanical stirring and ultrasonic wave stirring are conducted for a certain time until the mixture is mixed evenly, and electroplate liquid is obtained; a cathode electrode and an anode electrode are placed into an electroplating bath, a certain space between the electrodes, temperature, impulse frequency, pulse duty factor, deposition period and average current density are kept, pulse electroplating is conducted at a certain stirring speed, and after electroplating, washing and drying are conducted, and the Ni-Cr-PTFE composite coating is obtained, wherein a pretreated matrix serves as the cathode electrode, and a platinum sheet or graphite serves as the anode electrode. Due to the fact that the PTFE and Cr are added, the antifriction performance and hardness of the coating are obviously improved, the process procedure is simple, the equipment investment is low, and the method is environmentally friendly and economical.