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Method for preparing stephanoporate silicon/DPP photoelectricity composite material

A composite material and porous silicon technology, applied in photovoltaic power generation, semiconductor/solid-state device manufacturing, circuits, etc., can solve the problem of low photovoltaic performance, achieve the effect of improving charge separation efficiency, simple process, and low equipment requirements

Inactive Publication Date: 2009-09-02
ZHEJIANG UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

At present, most studies on porous silicon / organic compounds focus on luminescence, and there are few studies on the photovoltaic properties of porous silicon / organic compound materials.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

preparation example Construction

[0026] Preparation of DPP Saturated Solution Containing Trifluoroacetic Acid

[0027] (1) Add 0.98g (2.5mmol) PTDA, 1.37ml (10mmol) aniline, 0.5g anhydrous zinc acetate to 10ml quinoline, mix well and place in N 2 Under protection, react at 185°C for 8 hours, cool and filter to obtain the initial product;

[0028] (2) The initial product is first boiled and washed with 5% NaOH solution until the washing liquid has no obvious green color, then washed with deionized water until neutral, finally washed three times with absolute ethanol, and dried to obtain a reddish-brown solid;

[0029] (3) The reddish-brown solid was sublimated in vacuum and solidified to obtain a dark red needle-like crystal product, which was pure DPP, and the yield was 78.2%.

[0030] (4) Dissolve excess DPP in N,N-dimethylformamide (DMF) to form a suspension, and then add 0.5ml of 0.1mol / L trifluoroacetic acid dropwise to obtain saturated DPP containing trifluoroacetic acid. solution, its solvent is N, N-...

Embodiment 1

[0033] 1. Wash and degrease the boron-doped p-type (111) monocrystalline silicon wafer, and perform ultrasonic treatment in acetone, ethanol and deionized water for 10 minutes, and dry;

[0034] 2. Treat the dried single crystal silicon wafer with 10% hydrofluoric acid to remove SiO on the surface 2 , sputtering a layer of gold film with a thickness of 50nm on the back of the processed single crystal silicon wafer;

[0035] 3. Under the condition of energization, the monocrystalline silicon chip covered with gold film is used as the anode, and the platinum sheet is used as the cathode, and placed in a mixed solution of hydrofluoric acid and ethanol (the mass percentage of HF is 20%) for electrochemical Corrosion for 10 minutes, where the current density is 5mA / cm 2 ;

[0036] 4. Under the condition of energization, the corroded single crystal silicon wafer is used as the cathode, and the platinum wafer is used as the anode, placed in a DPP saturated solution containing trifl...

Embodiment 2

[0038] 1. Wash and degrease the boron-doped p-type (111) monocrystalline silicon wafer, and perform ultrasonic treatment in acetone, ethanol and deionized water for 10 minutes, and dry;

[0039] 2. Treat the dried single crystal silicon wafer with 10% hydrofluoric acid to remove SiO on the surface 2 , sputtering a layer of gold film with a thickness of 50nm on the back of the processed single crystal silicon wafer;

[0040] 3. Under the condition of energization, the monocrystalline silicon chip covered with gold film is used as the anode, and the platinum sheet is used as the cathode, and placed in a mixed solution of hydrofluoric acid and ethanol (the mass percentage of HF is 20%) for electrochemical Corrosion for 60 minutes, where the current density is 5mA / cm 2 ;

[0041] 4. Under the condition of energization, the corroded single crystal silicon wafer is used as the cathode, and the platinum wafer is used as the anode, placed in a DPP saturated solution containing trifl...

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Abstract

The invention discloses a method for preparing porous silicon / DPP photoelectrical compound material, comprising: washing off the oil stain on monocrystalline silicon wafer, carrying out ultrasonic treatment on the monocrystalline silicon wafer in acetone, alcohol and deionized water respectively, then drying; washing SiO2 on surface of the dried monocrystalline silicon wafer with hydrofluoric acid, sputtering a gold film on the back of the treated monocrystalline silicon wafer; under power-on state, putting the monocrystalline silicon wafer coated with gold film and a platinum sheet in electrolyte to carry out electrochemical corrosion, respectively as anode and cathode; under power-on state, by using the monocrystalline silicon wafer as the cathode and the platinum sheet as anode after the corrosion, immerging the two in DPP saturated solution containing trifluoroacetic acid to carry out electrochemical deposition, vacuum-drying the monocrystalline silicon wafer deposited with DPP. The manufacturing method according to the invention has simple procedure; the porous silicon can match with DPP energy level structure; thus, the porous silicon / DPP photoelectrical compound material can be widely applied in photovoltaic devices field.

Description

technical field [0001] The invention relates to the technical field of photoelectric composite materials, in particular to a method for preparing a porous silicon / DPP photoelectric composite material. Background technique [0002] Since Canham (Appl. Phys. Lett., 1990, 57: 1046) discovered the strong visible photoluminescence of porous silicon (PS) at room temperature in 1990, the research on porous silicon has aroused great interest of researchers. , Porous silicon is considered to be used in optoelectronic integration (Mater. Thin Solid Films 2005, 487: 170) and other fields have the potential of application. [0003] Porous silicon has a unique microporous structure, huge specific surface area, and strong adsorption capacity, making it a good carrier for organic molecules. Using porous silicon to embed organic matter to change the photoelectric performance of porous silicon is a problem worth exploring. Using porous silicon as a template to add organic matter to it has...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): H01L51/48
CPCY02E10/549
Inventor 陈红征刘楠施敏敏杨立功吴刚汪茫
Owner ZHEJIANG UNIV