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Preparation method of high-performance carbon molecular sieve for separating carbon dioxide/methane

A carbon dioxide and carbon molecular sieve technology, applied in separation methods, chemical instruments and methods, methane capture, etc., to achieve the effects of increasing adsorption capacity, improving efficiency, and reducing costs

Inactive Publication Date: 2014-04-02
UNIV OF SCI & TECH BEIJING
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] The present invention is aimed at CO 2 / CH 4 Problems existing in carbon molecular sieves for separation, provide a preparation method that can make agricultural wastes be used with high value, and obtain carbon molecular sieves with high adsorption capacity and high adsorption selectivity for carbon dioxide / methane

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0020] After drying, the corncobs are crushed to a length of about 1 cm, mixed and kneaded with a binder at a mass ratio of 1:1, and then extruded into a column shape of φ0.5 cm×1 mm. Carbonize at 500°C for 1 hour under a nitrogen atmosphere with a programmed temperature rise rate of 5°C / min. 2 CO 3 and a small amount of ethanol in an alkaline solution for 4 hours, open the mouth and dry it in a vacuum drying oven at 120°C, then put it into a closed crucible with small holes, that is, a semi-closed system, and place it in a muffle furnace under a static air atmosphere without an atmosphere. Or program the temperature in a tube furnace to 600°C for 1 hour, then continue to heat up to 800°C for 45 minutes at a rate of 5°C / min, then cool to room temperature naturally, take it out and wash with water until neutral. The activated product was soaked in diethanolamine solution for 4 hours at room temperature, dried in a vacuum oven, placed in a microwave oven, and programmed to heat...

Embodiment 2

[0022] After the tobacco rod is dried, it is crushed to a length of about 1 cm, mixed and kneaded with a binder at a mass ratio of 1.5:1, and then extruded into a column shape of φ0.5 cm×1 mm. Carbonize at 400°C for 1 hour under a nitrogen atmosphere with a programmed temperature rise rate of 5°C / min. 2 CO 3and a small amount of ethanol in an alkaline solution for 4 hours, open the mouth and dry it in a vacuum oven at 120°C, then put it into a semi-closed system as above, and heat it up to a constant temperature of 600°C in a muffle furnace or tube furnace under a static air atmosphere. After 1h, continue to heat up to 800°C for 45min at a constant temperature of 5°C / min, then cool naturally to room temperature, take it out and wash with water until neutral. The activated product was soaked in diethanolamine solution at room temperature for 4 hours, after drying, the sample was placed in a microwave oven, and the temperature was programmed to 500°C under a nitrogen atmosphere...

Embodiment 3

[0024] After the coconut shell is dried, it is crushed to a length of about 1cm, mixed with a binder at a mass ratio of 1.5:1 and kneaded, and then extruded into a column shape of φ0.5cm×1mm. Carbonize at 500°C for 1 hour under a nitrogen atmosphere, with a programmed temperature rise rate of 5°C / min. 2 CO 3 and a small amount of ethanol in an alkaline solution for 4 hours, open the mouth and dry it in a vacuum oven at 120°C, then put it into a semi-closed system as above, and heat it up to a constant temperature of 500°C in a muffle furnace or tube furnace under a static air atmosphere. After 1h, continue to heat up to 750°C for 1h at a constant temperature at a rate of 5°C / min, then cool down to room temperature naturally, take it out and wash with water until neutral. The activated product was soaked in diethanolamine solution at room temperature for 4 hours, after drying, the sample was placed in a microwave oven, and the temperature was programmed to rise to 400°C for 1 ...

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Abstract

The invention provides a preparation method of a carbon molecular sieve has high adsorptive selectivity and high adsorption capacity for CO2 / CH4 by using agricultural wastes as a raw material. The preparation method specifically comprises the steps of forming, carbonizing, activating and modifying. Main pore diameters of the obtained carbon molecular sieve are distributed between 0.3nm and 0.4nm, the specific surface area of the obtained carbon molecular sieve reaches 2400-2800m<2>.g<-1>, the carbon molecular sieve is high in CO2 adsorption capacity of 75-85mL.g<-1> at a normal temperature and normal pressure, and the equilibrium adsorption selectivity coefficient alpha (CO2 / CH4) of carbon dioxide and methane reaches a range of 65-73. According to the preparation method, the adsorption capacity of the carbon molecular sieve is increased, and the gas separation coefficient of the carbon molecular sieve and the CO2 / CH4 is increased by using a modifying method; the preparation method has wide application prospect in a gas separation technology.

Description

technical field [0001] The invention belongs to the field of comprehensive utilization of energy, and relates to a preparation method of a high-performance carbon molecular sieve for separating carbon dioxide / methane, in particular to high-value utilization of agricultural waste and a preparation method of a high-performance carbon molecular sieve. Background technique [0002] With the shortage of fossil energy and the increasing pressure of environmental pollution, how to use clean energy to replace gasoline, coal and other fuels has become an urgent problem to be solved. Methane / carbon dioxide mixtures are widely found in resources such as coalbed methane, oilfield gas, landfill gas, and biogas. As an efficient and clean energy source, if methane can be separated from it and concentrated and utilized, it will not only generate huge economic benefits, but also make an important contribution to environmental protection. In addition, CO 2 As a "potential carbon resource", ...

Claims

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Application Information

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IPC IPC(8): B01J20/22B01J20/30C01B31/08C01B31/12B01D53/02C01B32/306C01B32/348
CPCY02C20/20Y02C10/08Y02C20/40Y02P20/151
Inventor 黄冬华周花蕾董彬孙长艳刘世香
Owner UNIV OF SCI & TECH BEIJING