Nitride ceramic-microcrystalline glass composite material and preparation method thereof
A technology of nitride ceramics and glass-ceramics, applied in the field of inorganic composite materials, can solve the problems of low output, long cycle, poor repeatability, etc., achieve simple and efficient process, easy components, improved thermal shock resistance and ablation resistance Effect
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Embodiment 1
[0024] A method for preparing a nitride ceramic-glass-ceramics composite material, comprising the steps of:
[0025] 1) Weigh 68% of raw material silicon nitride and 32% of boron oxide powder according to mass percentage, wherein boron oxide is obtained by dehydration and transformation of boric acid, and the quality of boron oxide is converted according to 56.3% of the mass of boric acid; the weighed silicon nitride Put boric acid and boric acid into the agate tank, add agate balls according to the ball-to-material ratio of 2:1; then add grinding aid acetone or n-hexane; mix on a planetary ball mill for 4 hours to obtain a slurry;
[0026] 2) drying the slurry at 80-90°C for 2-4 hours, removing the ball milling aid, grinding, and passing through a 100-mesh standard sieve to obtain a solid powder;
[0027] 3) Put the solid powder obtained in step 2) into a graphite mold coated with boron nitride on the inner wall. After the mold is loaded, put it into a hot-press furnace, keep...
Embodiment 2
[0030] The difference with the preparation method of nitride ceramics-glass-ceramics composite material in embodiment 1 is:
[0031] The raw material is composed of 57wt.% silicon nitride and 43wt.% boron oxide powder; boron oxide is obtained by dehydration and conversion of boric acid, and the mass of boron oxide is obtained by converting 56.3% of the mass of boric acid.
[0032] Other processes are the same as in Example 1.
[0033] figure 1 a is the phase diagram of the product obtained in this embodiment; it can be seen that its structure is composed of fine-crystalline boron nitride and glass-ceramics.
Embodiment 3
[0035] The difference with the preparation method of nitride ceramics-glass-ceramics composite material in embodiment 1 is:
[0036] The raw material is composed of 50wt.% silicon nitride and 50wt.% boron oxide powder; boron oxide is obtained by dehydration and conversion of boric acid, and the mass of boron oxide is obtained by converting 56.3% of the mass of boric acid.
[0037] Other processes are the same as in Example 1.
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