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A method for preparing calcium fluoride from lime calcined residue

A calcium fluoride, calcining technology, applied in the direction of calcium/strontium/barium fluoride, ammonium chloride, silicon oxide, etc., can solve the problem of high impurity content in the final product of calcium fluoride, difficult to control the purity of calcium oxide, and difficult to control the reaction process and other problems, to achieve the effect of comprehensive utilization of waste residue, easy control of the reaction process and high production efficiency

Inactive Publication Date: 2018-06-01
淄博志华环保科技有限公司 +2
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] Patent application number 200610106969.2 discloses a method for producing calcium oxide. In this application, calcium fluorosilicate is produced by reacting by-product fluorosilicic acid with calcium oxide, and calcium fluorosilicate is heated to produce calcium fluoride. The raw material calcium oxide used is The purity is difficult to control, and its impurity content is high, so that the impurity content in the final product of calcium fluoride is high, and there is a phenomenon of silicon exceeding the standard, and there will be bumping phenomenon in the reaction between fluosilicic acid and calcium oxide, and the reaction process is difficult to control

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0029] A method for preparing calcium fluoride by utilizing lime calcined residue, comprising the following steps:

[0030] 1) First add 30% fluosilicic acid solution into the reaction tank, and then add ammonia water with a mass fraction of 17% while stirring at a stirring speed of 20r / min. The speed of adding ammonia water is 20L / min. React for 1 hour at 50°C, where the molar ratio of ammonia water to fluorosilicic acid is 4.2;

[0031] 2) Pass the slurry obtained in step 1) into the filter tank, vacuum filter, the filter cake is a solid mixture of fluorosilicate, and the filtrate enters the fluorosilicate absorption device, and continues to recover fluorosilicate;

[0032] 3) Put the fluorosilicate solid mixture obtained in step 2) into the reaction kettle, add ammonia water with a mass fraction of 9%, stir while adding, the stirring speed is 40r / min, react for 1h, and wait until the pH of the slurry reaches 7.0, end the reaction, wherein the molar ratio of fluorosilicate ...

Embodiment 2

[0041] A method for preparing calcium fluoride by utilizing lime calcined residue, comprising the following steps:

[0042] 1) First add 30% fluosilicic acid solution into the reaction tank, and then add ammonia water with a mass fraction of 17% while stirring at a stirring speed of 20r / min. The speed of adding ammonia water is 20L / min. React for 1 hour at 50°C, where the molar ratio of ammonia water to fluorosilicic acid is 4.2;

[0043] 2) Pass the slurry obtained in step 1) into the filter tank, vacuum filter, the filter cake is a solid mixture of fluorosilicate, and the filtrate enters the fluorosilicate absorption device, and continues to recover fluorosilicate;

[0044] 3) Put the fluorosilicate solid mixture obtained in step 2) into the reaction kettle, add ammonia water with a mass fraction of 9%, stir while adding, the stirring speed is 40r / min, react for 1h, and wait until the pH of the slurry reaches 7.0, end the reaction, wherein the molar ratio of fluorosilicate ...

Embodiment 3

[0053] A method for preparing calcium fluoride by utilizing lime calcined residue, comprising the following steps:

[0054] 1) First add 30% fluosilicic acid solution into the reaction tank, and then add ammonia water with a mass fraction of 25% while stirring at a stirring speed of 30r / min. The speed of adding ammonia water is 30L / min. Reaction at 60°C for 2 hours, wherein the molar ratio of ammonia water to fluorosilicic acid is 5.0;

[0055] 2) Pass the slurry obtained in step 1) into the filter tank, vacuum filter, the filter cake is a solid mixture of fluorosilicate, and the filtrate enters the fluorosilicate absorption device, and continues to recover fluorosilicate;

[0056] 3) Put the fluorosilicate solid mixture obtained in step 2) into the reaction kettle, add ammonia water with a mass fraction of 10%, stir while adding, the stirring speed is 60r / min, and react for 2h, until the pH of the slurry reaches 7.5, end the reaction, wherein the molar ratio of fluorosilicat...

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Abstract

The invention relates to a method for preparing calcium fluoride from lime calcination residues. Firstly, a fluosilicic acid solution reacts with ammonia water to produce a fluorosilicate solid mixture, and the obtained fluorosilicate solid mixture reacts with ammonia water to produce an ammonium fluoride solution and a white carbon black filter cake; lime calcination residues react with by-product hydrochloric acid to produce a calcium chloride solution, and finally, the calcium chloride solution reacts with an ammonium fluoride solution to produce calcium fluoride. Compared with the prior art, the method has the characteristics that the cost is low, waste use of the lime calcination residues can be realized, and the quality of white carbon black and calcium fluoride products is high.

Description

technical field [0001] The invention relates to the technical field of calcium fluoride preparation, in particular to a method for preparing calcium fluoride by using lime calcined residue. Background technique [0002] Calcium fluoride is an important raw material in the fluorine chemical industry, which affects the development of fluorine chemical industry and related industries. It is widely used in chemical and metallurgical industries, and has an important impact on national security, national economy and social development. At present, in order to reduce the production cost of calcium fluoride and realize the sustainable development of fluorine resources, there have been some methods of using the by-product fluosilicic acid produced by phosphate fertilizer plants and hydrofluoric acid plants as raw materials to produce calcium fluoride. Through these methods The reuse of the by-product fluorosilicic acid is realized, and the cost is reduced to a certain extent, but the...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C01F11/22C01C1/16C01F11/28C01B33/12
CPCC01B33/12C01C1/164C01F11/22C01F11/28C01P2006/12C01P2006/80
Inventor 邹逸根侯新涛
Owner 淄博志华环保科技有限公司