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A method for preparing ultrafine tungsten-copper composite powder

A composite powder, tungsten copper technology, applied in the field of alloy materials, can solve the problems of high cost, complicated process, easy introduction of impurities, etc., and achieve the effect of low cost and simple operation

Active Publication Date: 2020-04-10
UNIV OF SCI & TECH BEIJING
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

At present, tungsten-copper composite powder is mainly prepared by hydrogen reduction of tungsten-copper oxide, but to prepare ultra-fine tungsten-copper composite powder, special pretreatment of raw materials is required, such as sol-gel method to obtain composite oxide, Or high-energy ball milling, these processes are complex, costly, and easy to introduce impurities

Method used

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Examples

Experimental program
Comparison scheme
Effect test

example 1

[0013] Example 1: To prepare W-30% Cu alloy, the mass ratio of tungsten to copper in ammonium tungstate and copper nitrate is uniformly mixed according to 7:3. Then put this raw material into a high-temperature furnace under an air atmosphere, heat up to 400° C. with the furnace, keep it warm for 4 hours, and then cool it in an air atmosphere. Carbon distribution follows the following rules: WO 3 and for restoring WO 3 The molar ratio of carbon black is 1:2; the molar ratio of CuO and carbon black used to reduce CuO is 1:0.5. After uniform mixing, react at 600°C for 2 hours under an argon atmosphere, and then react at 1000°C for 2 hours. hours, and then cooled under argon atmosphere to obtain W, Cu and a small amount of WO 2 mixture. Then the carbothermal pre-reduced product was kept at 800°C for 4 hours in a hydrogen atmosphere, and cooled to room temperature in a hydrogen atmosphere to obtain a tungsten-copper composite powder with a particle size of less than 200nm.

example 2

[0014] Example 2: To prepare a W-10% Cu alloy, the mass ratio of tungsten to copper in ammonium tungstate and copper nitrate is uniformly mixed according to 90:10. Then put the raw material into a high-temperature furnace and heat it up to 500° C. in an air atmosphere, keep it warm for 4 hours, and then cool it in an air atmosphere. Carbon distribution follows the following rules: WO 3 and for restoring WO 3 The molar ratio of carbon black is 1:2.1; the molar ratio of CuO and carbon black used to reduce CuO is 1:0.5. After uniform mixing, react at 600°C for 2 hours under an argon atmosphere, and then react at 1000°C 2 hours, and then cooled under argon atmosphere to obtain W, Cu and a small amount of WO 2 mixture. Then, the carbothermally pre-reduced product is kept at 850° C. for 2 hours in a hydrogen atmosphere, and cooled in a hydrogen atmosphere to obtain a tungsten-copper composite powder with a particle size of less than 200 nm.

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Abstract

The invention relates to a method for preparing ultrafine tungsten-copper alloy powder, and belongs to the field of alloy materials. Ammonium tungstate and copper nitrate are burdened, ground and mixed according to the required copper content to obtain a uniformly-mixed powder raw material; the powder raw material is calcined under an air atmosphere, temperature preservation is carried out for a certain period of time, heat preservation is finished, cooling is performed, and corresponding oxide powder is obtained; then the oxide powder and carbon black less than the theoretical ratio are burdened according to a certain molar ratio, carbon thermal pre-reducing is carried out under an argon atmosphere, and powder containing a small amount of WO2 most W and Cu is obtained; and the powder obtained after carbon thermal reducing under a hydrogen atmosphere is subjected to deep deoxygenation to obtain ultrafine tungsten-copper composite powder. By using the technological process, the tungsten-copper composite powder with the crystal grain smaller than 200 nm and the uniformly-distributed size can be obtained. The method is simple in operation and low in cost and easily achieves industrialized operation. By means of the scheme, the method can also be used for preparing ultrafine molybdenum-copper composite powder.

Description

technical field [0001] The invention belongs to the field of alloy materials and discloses a method for preparing ultrafine tungsten-copper composite powder, in particular to a method for preparing tungsten-copper composite powder by combining carbon black and hydrogen in two-stage reduction. Background technique [0002] Tungsten-copper alloy not only has the high hardness and high melting point of tungsten, but also has the high electrical and thermal conductivity of copper. Among them, tungsten has a high melting point (3410°C) and a high density (19.34g / cm 3 ); Copper has excellent electrical and thermal conductivity, tungsten-copper alloy (composition generally ranges from WCu7-WCu50) has uniform microstructure, high temperature resistance, high strength, arc ablation resistance, and high density; moderate electrical and thermal conductivity, widely used in military high temperature resistance Materials, electrical alloys for high-voltage switches, electrodes for elect...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B22F9/22
CPCB22F9/22
Inventor 张国华刘军凯吉鑫鹏焦树强周国治
Owner UNIV OF SCI & TECH BEIJING