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Neutralization treatment method of nickel and cobalt precipitation post-liquid

A treatment method, nickel deposition technology, applied in the improvement of process efficiency, recycling of waste collectors, lithium carbonate;/acid carbonate, etc., can solve problems such as easy crystallization and difficult process

Inactive Publication Date: 2020-04-07
甘肃睿思科新材料有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0003] The purpose of the present invention is to provide a neutralization treatment method for nickel-cobalt after-liquid, so as to separate nickel-cobalt from waste batteries, and different from the general use of sodium hydroxide for neutralization, the after-liquid contains extremely high sulfuric acid Sodium, easy to crystallize, causing difficult problems in the process

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0014] 1) Calcining the nickel-cobalt lithium manganese oxide positive electrode material at 300-600°C, the calcination residence time is about 5-10min; prepare 200-250g / L dilute sulfuric acid solution, add the calcined positive electrode material, the solid-liquid ratio is 100-120g: 1L, raise the temperature to 90-100°C, and react for 2 hours to obtain a low-manganese leaching solution and leaching residue.

[0015] 2) Raise the temperature of the low-manganese leaching solution to 60°C, slowly add solid oxalic acid, the amount added is 1.4 times the mass required by the theory of nickel-cobalt precipitation, and react for 2 hours to obtain the nickel-cobalt oxalate solid and the solution after nickel-cobalt precipitation, after nickel-cobalt precipitation The nickel content in the liquid is less than 0.2g / L, the cobalt content is less than 0.4g / L, and the manganese content is less than 0.01g / L.

[0016] 3) Neutralize the solution after precipitation of nickel and cobalt with...

Embodiment 2

[0018] 1) Calcining the nickel-cobalt lithium manganese oxide positive electrode material at 300-600°C, the calcination residence time is about 5-10min; prepare 200-250g / L dilute sulfuric acid solution, add the calcined positive electrode material, the solid-liquid ratio is 100-120g: 1L, raise the temperature to 90-100°C, and react for 2 hours to obtain a low-manganese leaching solution and leaching residue.

[0019] 2) Raise the temperature of the low-manganese leaching solution to 70°C, slowly add solid oxalic acid, the amount added is 1.4 times the mass required by the theory of nickel-cobalt precipitation, and react for 1 hour to obtain nickel-cobalt oxalate solid and nickel-cobalt-precipitated liquid, after nickel-cobalt precipitation The nickel content in the liquid is less than 0.2g / L, the cobalt content is less than 0.4g / L, and the manganese content is less than 0.01g / L.

[0020] 3) Neutralize the solution after precipitation of nickel and cobalt with solid calcium hyd...

Embodiment 3

[0022] 1) Calcining the nickel-cobalt lithium manganese oxide positive electrode material at 300-600°C, the calcination residence time is about 5-10min; prepare 200-250g / L dilute sulfuric acid solution, add the calcined positive electrode material, the solid-liquid ratio is 100-120g: 1L, raise the temperature to 90-100°C, and react for 2 hours to obtain a low-manganese leaching solution and leaching residue.

[0023] 2) Raise the temperature of the low-manganese leaching solution to 90°C, slowly add solid oxalic acid, the amount of which is 1.4 times the mass required for the precipitation of nickel and cobalt theory, and react for 1 hour to obtain the nickel-cobalt oxalate solid and the liquid after precipitation of nickel and cobalt, after precipitation of nickel and cobalt The nickel content in the liquid is less than 0.2g / L, the cobalt content is less than 0.4g / L, and the manganese content is less than 0.01g / L.

[0024] 3) Neutralize the solution after precipitation of nic...

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PUM

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Abstract

The invention discloses a neutralization treatment method of a nickel and cobalt precipitation post-liquid. The method comprises the following operating steps of: preparing a low-manganese leaching solution from a lithium nickel-cobalt-manganese cathode material; rising the temperature of the low-manganese leaching solution to 60-90 DEG C; slowly adding oxalic acid solid, wherein the adding amountis 1.4-1.7 times of the theoretically needed mass of nickel and cobalt precipitation, a nickel and cobalt oxalate solid and nickel and cobalt precipitation liquid are obtained through filtering afterreaction for 1-2 hours, and in the nickel and cobalt precipitation liquid, the content of nickel is smaller than 0.2 g / L, the content of the cobalt is smaller than 0.4 g / L, and the content of the manganese is smaller than 0.01 g / L; and neutralizing the nickel and cobalt precipitation post-liquid with calcium hydroxide, then performing treating with activated carbon to remove residual nickel-cobalt-manganese impurities, and finally adding sodium carbonate for lithium precipitation to obtain industrial-grade lithium carbonate. The method disclosed by the invention is beneficial to separation ofnickel and cobalt elements in the waste battery.

Description

technical field [0001] The invention belongs to the technical field of nickel-cobalt-lithium-manganese-oxide positive-electrode material treatment, and in particular relates to a method for neutralizing the solution after depositing nickel and cobalt. Background technique [0002] With the continuous increase of human consumption of electronic products, more and more scrap batteries are produced. Waste lithium-ion batteries contain high-value metals such as cobalt, nickel, iron, aluminum, and copper. It is of great significance to recycle high-value metals in metals. Contents of the invention [0003] The purpose of the present invention is to provide a neutralization treatment method for nickel-cobalt after-liquid, so as to separate nickel-cobalt from waste batteries, and different from the general use of sodium hydroxide for neutralization, the after-liquid contains extremely high sulfuric acid Sodium is easy to crystallize, which causes the problem of difficult process...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C22B23/00C22B26/12C22B1/00H01M10/54C01D15/08
CPCC01D15/08C22B1/005C22B23/0461C22B26/12H01M10/54Y02W30/84Y02P10/20
Inventor 陈世鹏计彦发多金鹏温浩浩
Owner 甘肃睿思科新材料有限公司