Organosilicon polymer and preparation method thereof, and adhesive and application thereof
A silicone and polymer technology, applied in the field of silicone polymers and their preparation, can solve the problems of slow initial curing speed, poor storage stability, and application limitations of single-component dealcoholized adhesives, and achieve shortened packaging waiting time, Ease of storage and the effect of improving the initial bonding strength
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[0041] In another typical embodiment of the present application, a preparation method of the aforementioned organosilicon polymer is provided, which is characterized in that the preparation method includes: step S1, combining polysiloxane a with R 13 Si(R 7 ) 3-y (OR 8 ) y Carry out addition reaction; Or step S1 ', polysiloxane a and Si(R 7 ) 4-x (OR 8 ) x Carry out condensation reaction under alkaline condition, obtain the organosilicon polymer of general structural formula I; The structural general formula of above-mentioned polysiloxane a is as follows: Among them, R 13 is H or vinyl, R 1 , R 2 , R 3 , R 4 , R 5 , R 6 , R 7 , R 8 , m, n, p, y, z are the same as R in the general formula I 1 , R 2 , R 3 , R 4 , R 5 , R 6 , R 7 , R 8 , m, n, p, y, z, in step S1, R 12 For H, R 4 is vinyl; R 12 For vinyl, R 4 is H; in step S1', R 4 For hydroxyl.
[0042]In order to facilitate those skilled in the art to synthesize the above-mentioned organosilicon p...
Embodiment 1
[0057] When adding 100 parts into a mixing container equipped with stirring blades at 25°C, the viscosity is 3500mPa·s, and the structural formula is (CH 2 =CH)[(CH 3 ) 2 SiO] 12 [(CH 2 =CH)(CH 3 )SiO] 2 Si(CH 3 ) 2 (CH=CH 2 ) of polydimethylsiloxane (vinyl content is 0.8wt%), 9 parts of trimethoxysilylethylenetetramethyldisiloxane, 0.01 part of platinum vinyl silicon with a mass fraction of 0.7% The oxane complex was stirred at 40°C for 3h to obtain the organosilicon polymer 1.
[0058] Put 100 parts of α, ω-dihydroxypolydimethylsiloxane with a viscosity of 20000mpa·s at 25°C, 10 parts of simethicone oil with a viscosity of 500mpa·s, and 100 parts of light calcium carbonate into the planetary mixer In the process, start stirring and dispersing, dehydrate at 120~140°C, -0.09~-0.1MPa vacuum condition for 2~4 hours, then cool down to below 50°C. Add 3.5 parts of methyltrimethoxysilane, add 3 parts of the above silicone polymer 1, 3 parts of diisopropyl di(acetoacetate)...
Embodiment 2
[0060] When adding 100 parts into a mixing container equipped with stirring blades, the viscosity is 300mPa·s at 25°C, and the structural formula is (H)[(CH 3 ) 2 SiO] 10 [(CH 3 )(H)SiO] 4 Si(CH 3 ) 2 (H) polydimethylsiloxane (hydrogen content is 0.1wt%), 16 parts of vinyltrimethoxysilane, 0.01 part of platinum mass fraction is 0.7% platinum·vinylsiloxane complex, in Stir at 30-40°C for 2-3 hours to obtain organosilicon polymer 2.
[0061] 100 parts of trimethoxysilane-terminated polydimethylsiloxane with a viscosity of 50000mpa·s at 25°C, 20 parts of simethicone oil with a viscosity of 100mpa·s, 80 parts of light calcium carbonate, heavy calcium carbonate Put 40 parts into the planetary mixer, start stirring and dispersing, dehydrate at 120~140℃, -0.09~-0.1MPa vacuum condition for 2~4 hours, then cool down to below 50℃. Add 3.5 parts of methyltrimethoxysilane, 1.5 parts of the above silicone polymer 2, 3 parts of isopropyl titanate modified with ethyl acetoacetate, and...
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