Lithium ion quaternary positive electrode material, preparation method thereof and lithium ion battery
A technology for lithium ion batteries and positive electrode materials, which is applied in the direction of positive electrodes, battery electrodes, secondary batteries, etc., can solve the problems of poor safety and cycle performance, decreased material structure stability, etc., and improve cycle performance and cycle life. , to avoid loosening and pulverization, the effect of excellent cycle performance
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[0038] According to a first aspect of the present invention, the present invention provides a kind of preparation method of lithium-ion battery quaternary cathode material, comprises the following steps:
[0039] Co-precipitate the mixed solution of soluble nickel salt, soluble cobalt salt, and soluble manganese salt, aluminum hydroxide colloidal solution and alkali solution to prepare a quaternary transition metal hydroxide precursor. The quaternary transition metal hydroxide precursor The body and the lithium source are mixed and sintered to obtain a quaternary positive electrode material for a lithium-ion battery.
[0040] In the present invention, the quaternary transition metal hydroxide precursor is prepared by co-precipitation method by using aluminum hydroxide colloidal solution instead of soluble aluminum salt, soluble nickel salt, soluble cobalt salt and soluble manganese salt. Controlled, the quaternary transition metal hydroxide precursor with uniform distribution ...
Embodiment 1
[0076] This embodiment provides a quaternary cathode material for a lithium-ion battery, which is prepared according to the following steps:
[0077] (1) configure the first solution: take nickel sulfate hexahydrate, manganese sulfate monohydrate, and cobalt sulfate heptahydrate according to the molar ratio nickel: cobalt: manganese=0.88:0.06:0.03, utilize deionized water to dissolve, and configure to obtain mass concentration of 2mol / L transition metal salt solution, called the first solution;
[0078] (2) Configure the second solution: weigh aluminum nitrate nonahydrate and dissolve it in deionized water, then add concentrated ammonia water with a mass concentration of 25% into the aluminum salt solution drop by drop, and keep stirring, when pH=8-9 stop dripping concentrated ammonia water, and finally set the volume to the aluminum hydroxide concentration of 0.11mol / L, which is called the second solution;
[0079] (3) Preparation of quaternary transition metal hydroxide pre...
Embodiment 2
[0082] This embodiment provides a lithium-ion battery quaternary positive electrode material, the difference between its preparation method and embodiment 1 is that in step (4), when the hydroxide precursor and lithium hydroxide are mixed and sintered, 500 ℃ sintering for 3 hours, 850 ℃ sintering for 15 hours, and then the product was crushed and sieved to a D50 of 12 microns while cooling down.
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