Rare-earth doped spinel ferrite/aluminum-doped zinc oxide composite fiber and preparation method thereof
A technology of spinel ferrite and aluminum-doped zinc oxide, applied in the direction of inorganic raw material artificial filaments, etc., can solve the problems that have not yet been reported publicly on rare earth-doped spinel ferrite/ZAO composite fiber, and achieve the process The effects of controllable parameters and microstructure, convenient operation, and good mechanical and optical properties
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Embodiment 1
[0026] (1) Preparation of gel precursor: firstly dissolve basic nickel carbonate, cobalt nitrate, ferric nitrate, samarium oxide, and citric acid in deionized water, and Ni 2+ : Co 2+ : Fe 3+ The molar ratio of :Sm:organic acid is 0.6:0.4:1.9:0.1:8. Stir evenly, stir at room temperature for 15-20 hours, and form a gel precursor after dehydration under reduced pressure;
[0027] (2) The organogel precursor is spun into gel cellulose filaments by picking or spinning or spinning. The cellulose filaments are in the temperature range of 700 to 800 ℃, and after holding for 5 to 6 hours, they are naturally cooled to room temperature. Obtain rare earth doped spinel ferrite Ni 0.6 Co 0.4 Fe 1.9 Sm 0.1 O 4 Fiber, which is the core of composite fiber;
[0028] (3) Put zinc acetate dihydrate and aluminum trichloride hexahydrate into a mixed solvent of ethanolamine and glycol methyl ether, where the molar ratio of Al:Zn:solvent is 1:0.1:12, and the temperature is kept at 30°C 2 Dissolve and rea...
Embodiment 2
[0032] (1) Preparation of gel precursor: first dissolve nickel acetate, cobalt acetate, ferric nitrate, samarium oxide and lactic acid in deionized water, and Ni 2+ : Co 2+ : Fe 3+ The molar ratio of :Sm:organic acid is 0.7:0.3:1.8:0.2:7, stir evenly, and stir at room temperature for 12-15 hours, and form a gel precursor after dehydration under reduced pressure;
[0033] (2) The organogel precursor is spun into gel cellulose filaments by picking or spinning or spinning. The cellulose filaments are in the temperature range of 600-700°C, and after holding for 7 hours, they are naturally cooled to room temperature to obtain rare earths. Doped spinel ferrite Ni 0.7 Co 0.3 Fe 1.8 Sm 0.2 O 4 Fiber, which is the core of composite fiber;
[0034] (3) Put zinc acetate dihydrate and aluminum trichloride hexahydrate into the mixed solvent of ethanolamine and glycol methyl ether, the molar ratio of Al:Zn:organic solvent is 1:0.2:13, and the temperature is kept at 40℃ for 2 hours Dissolve and r...
Embodiment 3
[0038] The rare earth element is replaced with Ce, and the others are the same as in Example 1. The obtained composite fiber has a core diameter of 8-12 μm, a length of 400 μm-1m, and a coating thickness of 80-90 nm. The composite fiber has an attenuation of about 8dB in the 1-30GHz band and a bending strength of 1300-1700kg / cm 2 .
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