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Simple and convenient preparation method of copper-manganese compound oxide monolithic catalyst

A monolithic catalyst, composite oxide technology, applied in metal/metal oxide/metal hydroxide catalysts, physical/chemical process catalysts, chemical instruments and methods, etc., can solve the problem of low adhesion stability of active substances, preparation of Complex process and other problems, to achieve the effect of high mechanical stability, simple preparation process and low price

Inactive Publication Date: 2013-02-13
SOUTHEAST UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005]Technical problem: The purpose of the present invention is to solve the shortcomings of the current monolithic catalysts such as complicated preparation process and low adhesion stability of active substances on the monolithic carrier, and provide a A simple preparation method of a copper-manganese composite oxide monolithic catalyst for catalytic combustion purification of organic waste gas

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0021] (1) Preparation of slurry

[0022] Weigh 5 g pseudoboehmite powder, 2.5 g urea, 1.2476 g manganese nitrate solution (50% mass fraction), 0.8434 g Cu(NO 3 ) 2 ·3H 2 O, 1 ml CTAB and 1 ml Tween80 were placed in an 80 ml beaker, and 12.5 ml deionized water was added, placed on a magnetic stirrer, adjusted to pH 2 with nitric acid, and stirred vigorously for 1 h. After standing for 15 minutes, an aluminum sol slurry with high solid content, good fluidity, uniformity and stability, and containing active metal salts was formed.

[0023] (2) Coating of the carrier

[0024] Cordierite honeycomb ceramic carrier (composed of Mg 2 al 4 Si 5 o 18 , specifications: f 8′24 mm, square hole, hole density 400 cpsi, wall thickness 0.21 mm) after soaking in 50% acetic acid solution for 1 h and roasting at 600 °C for 2 h, immerse it in the above slurry and keep stirring Slowly take it out after 2 min. The excess liquid on the inner and outer walls of the channel was blown off by a...

Embodiment 2

[0028] (1) Preparation of slurry

[0029] Weigh 5 g pseudoboehmite, 3 g urea, 1.2482 g manganese nitrate solution (50% mass fraction), 0.8439 g Cu(NO 3 ) 2 ·3H 2 O, 1.5 ml CTAB and 2 ml Tween80 were placed in an 80 ml beaker, and 10 ml deionized water was added, placed on a magnetic stirrer, adjusted to pH 1.5 with nitric acid, and stirred vigorously for 1 h. After standing for 15 minutes, an aluminum sol slurry with high solid content, good fluidity, uniformity and stability, and containing active metal salts was formed.

[0030] (2) Coating of the carrier

[0031] The acid-etched pretreated cordierite ceramic carrier was immersed in the above slurry and kept stirring for 1 min, then slowly removed. The excess liquid on the inner and outer walls of the channel was blown off by air flow, turned over at room temperature for 1 h, left to stand for 18 h, then dried at 120 °C for 1 h, and then calcined at 500 °C for 3 h to obtain an alumina loading of 19.3 wt%. and a monolith...

Embodiment 3

[0035] (1) Preparation of slurry

[0036] Weigh 5 g pseudoboehmite, 2.5 g urea, 1.2475 g manganese nitrate solution (50% mass fraction), 0.8430 g Cu(NO 3 ) 2 ·3H 2O, 2 ml SDBS and 2 ml Tween20 were placed in an 80 ml beaker, and 10 ml deionized water was added, placed on a magnetic stirrer, adjusted to pH 1.5 with nitric acid, and stirred vigorously for 1 h. After standing for 15 minutes, an aluminum sol slurry with high solid content, good fluidity, uniformity and stability, and containing active metal salts was formed.

[0037] (2) Coating of the carrier

[0038] The acid-etched pretreated cordierite ceramic carrier was immersed in the above slurry and kept stirring for 2 min, then slowly removed. The excess liquid on the inner and outer walls of the channel was blown off by air flow, turned over at room temperature for 1 h, allowed to stand for 24 h, then dried at 150 °C for 2 h, and then calcined at 500 °C for 3 h to obtain an alumina loading of 19.9 wt%. and a monoli...

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PUM

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Abstract

The invention discloses a simple and convenient preparation method of a copper-manganese compound oxide monolithic catalyst, belonging to the technical field of catalytic technologies. The preparation method comprises the following steps of: mixing pseudoboehmite, urea, a surfactant, metal nitrate and deionized water; adjusting the pH value to 1.5-3 with nitric acid; stirring to obtain integral sol slurry which has high flowability, is uniform and stable and contains active metal salts; soaking a dichroite honeycomb carrier which is pretreated by acid etching into the slurry for 1-3 minutes; drying at 80-150 DEG C for 0.5-3 hours; and baking at 400-800 DEG C for 2-10 hours to obtain the monolithic catalyst. When used for catalyzing combustion and purification of xylene organic waste gases, the prepared monolithic catalyst has high catalytic activity. Meanwhile, the preparation method of the monolithic catalyst has the advantages of simple and convenient process, firm adhesion of active matters, low cost, contribution to industrial mass production, wide application prospect, and the like.

Description

technical field [0001] The invention relates to a simple monolithic catalyst preparation method, in particular to a simple preparation method of a copper-manganese composite oxide monolithic catalyst used for catalytic combustion purification of organic waste gas. Background technique [0002] A monolithic catalyst is an integrated catalyst with many narrow parallel channels neatly arranged, and usually consists of three parts: a monolithic carrier, a coating and an active component. The monolithic carrier is the basic skeleton of the catalyst. There are two types of common honeycomb ceramic carrier and metal carrier; the coating is used to increase the specific surface area of ​​the catalyst, and at the same time, it can also enhance the adhesion of the loaded active components on the monolithic carrier. Some coatings themselves also have Certain catalytic activity; the active component is the key part of the monolithic catalyst, which can provide the catalytic active sites...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J23/889B01D53/72B01D53/86
Inventor 吴东方李望兵边珊珊傅慧云冯翔马婧雯
Owner SOUTHEAST UNIV