Method for producing polyimide laminate and polyimide laminate
A technology of polyimide layer and pressed products, which is applied in the field of polyimide laminated products and its preparation, can solve the problems of reduced adhesion, reduced system vacuum, insufficient heat resistance, etc., and can inhibit thermal decomposition , Excellent heat resistance, high heat resistance effect
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Embodiment 1
[0125] In a 500 mL (internal volume) glass reactor equipped with a stirrer and nitrogen in / out tubes were placed 410.1267 g of N-methyl-2-pyrrolidone as a solvent. Then, 26.8886 g (0.2486 mol) of PPD and 73.1431 g (0.2486 mol) of s-BPDA were added thereto, and the mixture was stirred at 50° C. to provide a polyamic acid having a solid content of 18.21%, and an intrinsic viscosity of 0.65 dL / g solution. Then, 2.0006g (0.0061 mole, 2.5 mole % based on 100 mole % of the tetracarboxylic acid component, 2.0 wt % based on the total weight of the tetracarboxylic acid component and the diamine component, the same applies below) of phosphoric acid Triphenyl ester was added as a phosphorus compound to the resulting polyamic acid solution.
[0126] The polyamic acid solution was applied on a glass plate as a substrate with a bar coater. The resulting coating film was heated at 120°C for 10 minutes, 150°C for 40 minutes, 180°C for 60 minutes, 200°C for 10 minutes, 250°C for 10 minutes, ...
Embodiment 2
[0129] The same procedure as in Example 1 was carried out except that 5.0016 g (0.0153 mol, 6.2 mol %, 5.0 wt %) of triphenyl phosphate was added as a phosphorus compound. The results are shown in Table 2.
Embodiment 3
[0131] The same procedure as in Example 1 was carried out except that 15.0160 g (0.0460 mol, 18.5 mol%, 15.0 wt%) of triphenyl phosphate was added as a phosphorus compound. The results are shown in Table 2.
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Abstract
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