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A preparation method of polyamide quartz crystal chip assembled with polyelectrolyte

A technology of quartz crystals and polyelectrolytes, applied in polyamide coatings, material absorption weighing, coatings, etc., can solve problems that cannot represent the surface properties of polyamide nanofiltration membranes, and achieve the effect of ensuring modification

Inactive Publication Date: 2018-08-31
XI'AN UNIVERSITY OF ARCHITECTURE AND TECHNOLOGY
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Obviously, the commercialized quartz crystal chip cannot represent the surface performance of the actual polyamide nanofiltration membrane, which is the main reason why the dissipative quartz crystal microbalance technology has not been widely used in the field of membrane fouling.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

preparation example Construction

[0031] The preparation method of the polyamide quartz crystal chip assembled by polyelectrolyte of the present invention comprises the following steps:

[0032] 1) Substrate pretreatment: Soak the silica substrate in a sodium dodecyl sulfate solution with a temperature of 20-30°C and a mass concentration of 2-5% for 20-30 minutes, and then place it in ultrapure water , at a temperature of 20-30°C for 10-20 minutes, rinsed with ultrapure water and dried with nitrogen, and finally placed the silicon dioxide substrate under a UV lamp with a power of 30-40w and a wavelength of 185nm for 10- 30min, stand by;

[0033] 2) Generation of poly-L-lysine adsorption layer:

[0034]First prepare 4-hydroxyethylpiperazineethanesulfonic acid buffer solution and poly-L-lysine solution: dissolve 4-hydroxyethylpiperazineethanesulfonic acid in ultrapure water, the preparation concentration is 10mM, and the pH is 7 —7.5 4-hydroxyethylpiperazineethanesulfonic acid buffer solution, stand-by. Disso...

Embodiment 1

[0045] Soak the silicon dioxide substrate in a sodium lauryl sulfate solution with a temperature of 25°C and a mass concentration of 3% for 25 minutes, then place it in ultrapure water, and ultrasonically treat it at a temperature of 25°C for 10 minutes, and then Rinse fully with ultrapure water and blow dry with nitrogen, and finally place the silicon dioxide substrate under a UV lamp with a wavelength of 185nm and a power of 30w for 20min and set it aside.

[0046] 4-Hydroxyethylpiperazineethanesulfonic acid was dissolved in ultrapure water to prepare a 4-hydroxyethylpiperazineethanesulfonic acid buffer solution with a concentration of 10 mM and a pH of 7.4 for use. Poly-L-lysine hydrobromide was dissolved in 4-hydroxyethylpiperazineethanesulfonic acid buffer solution to obtain a poly-L-lysine solution with a concentration of 0.1 g / L, which was ready for use. Dissolve trimesoyl chloride and m-phenylenediamine in Isopar-G and N,N-dimethylacetamide respectively to obtain polym...

Embodiment 2

[0053] Soak the silicon dioxide substrate in a sodium lauryl sulfate solution with a temperature of 20°C and a mass concentration of 5% for 20 minutes, then place it in ultrapure water, and ultrasonically treat it at a temperature of 20°C for 20 minutes, and then Rinse fully with ultrapure water and blow dry with nitrogen, and finally place the silicon dioxide substrate under a UV lamp with a wavelength of 185nm and a power of 40w for 10min and set it aside.

[0054] 4-Hydroxyethylpiperazineethanesulfonic acid was dissolved in ultrapure water to prepare a buffer solution of 4-hydroxyethylpiperazineethanesulfonic acid with a concentration of 10 mM and a pH of 7 for use. Poly-L-lysine hydrobromide was dissolved in 4-hydroxyethylpiperazineethanesulfonic acid buffer solution to obtain a poly-L-lysine solution with a concentration of 0.3 g / L, which was ready for use. Dissolve trimesoyl chloride and m-phenylenediamine in Isopar-G and N,N-dimethylacetamide respectively to obtain poly...

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Abstract

The invention discloses a preparation method of a polyamide quartz crystal chip prepared from polyelectrolyte. The method includes the steps of preprocessing a silicon dioxide substrate through a physico-chemical method for use, modifying a poly-L-lysine adsorption layer on the clean silicon dioxide substrate through a dissipation type quartz crystal microbalance to obtain a chip modified by poly-L-lysine for use, sequentially coating the surface of the chip modified by poly-L-lysine with trimesoyl chloride and an m-phenylenediamine polymerization reaction solution through multi-cycle centrifugal spin coating, conducting constant-temperature heat treatment to obtain the polyamide quartz crystal chip prepared from polyelectrolyte, and recycling the silicon dioxide substrate through a polyamide quartz crystal chip cleaning solution. By means of the method, the nanoscale-thickness polyamide functional layer is uniformly bonded with the surface of the silicon dioxide substrate, and the polyamide quartz crystal chip prepared from polyelectrolyte is obtained; operation is easy, practicability is high, and the method can be widely used for analyzing surface adsorption behaviors and mechanisms of polyamide nanofiltration membrane pollution.

Description

technical field [0001] The invention belongs to the field of quartz crystal microbalance chip development, and in particular relates to a preparation method of a polyamide quartz crystal chip assembled with polyelectrolyte. Background technique [0002] Nanofiltration is a pressure-driven membrane separation process between reverse osmosis and ultrafiltration, and has become a hot research topic in membrane separation technology in the past three decades. Nanofiltration membranes mainly separate dissolved components through steric hindrance and electrostatic repulsion, and usually have a rejection rate of more than 90% for divalent and multivalent ions and organic compounds with a molecular weight greater than 200Da, while for monovalent ions and small molecular organic compounds. The retention rate is low. Therefore, the unique separation characteristics of nanofiltration membranes can realize the selective separation of different substances, and are widely used in water t...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): G01N5/02C08G69/32C09D177/10
CPCY02P20/582
Inventor 王磊王佳璇苗瑞张一吕永涛李珍贤刘婷婷王旭东
Owner XI'AN UNIVERSITY OF ARCHITECTURE AND TECHNOLOGY