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Sunflower flower seed husk adsorption material and preparation method thereof

A technology for sunflower seeds and adsorption materials is applied in the field of preparation of adsorption materials, which can solve the problems of environmental pollution, waste of resources and the like, and achieve the effects of simple preparation process, low cost and environmental friendliness.

Inactive Publication Date: 2019-02-26
李海鱼
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

At present, most of the sunflower husks are discarded or incinerated, which not only pollutes the environment but also wastes resources. However, the modification of sunflower husks into a low-cost heavy metal adsorption material will greatly improve the utilization efficiency of sunflower husks.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0026] Use sunflower seed shells to wash, mash, dry, grind, and pass through a 70-mesh sieve, and use 7% HNO 3 Reflux for 2 hours, then reflux with 3% NaOH for 1 hour, wash with water and dry; take 10 g of the obtained dried product and place it in a three-necked flask, add 20 ml of NaOH solution with a concentration of 2 mo / L and 60 ml of epichlorohydrin in sequence, and heat to reflux for 1 hour , filtered, cross-washed with acetone and water for 3-4 times, and dried at 60°C to obtain light yellow cross-linked cellulose; add a certain amount of cross-linked fiber to a three-necked bottle equipped with a reflux condenser and a stirrer Sulfonate, sodium 3-chloro-2-hydroxypropanesulfonate, 1mol / L dioxane aqueous solution and 1mol / L Na 2 CO 3 solution, stirred and reacted at 50°C for a certain period of time, and then the product was filtered out, and the product was washed three times with water and alcohol successively; after washing, it was vacuum-dried to obtain 2-hydroxy-3...

Embodiment 2

[0028] Use sunflower seed shells to wash, mash, dry, grind, and pass through a 70-mesh sieve, and use 9% HNO 3 Reflux for 3 hours, then reflux with 5% NaOH for 2 hours, wash with water and dry to obtain sunflower seed shell cellulose; take 20 g of the obtained cellulose and place it in a three-necked bottle, add 20 ml of NaOH solution with a concentration of 3 mo / L, 60 ml of ring Oxychloropropane, heated to reflux for 2 hours, filtered, cross-washed with acetone and water until neutral, dried at 80°C to obtain light yellow cross-linked cellulose; add a certain amount of The cross-linked cellulose, sodium 3-chloro-2-hydroxypropanesulfonate, 1mol / L dioxane aqueous solution and 1mol / L Na 2 CO 3 solution, shake it gently, stir and react under temperature control at 60°C for a certain period of time, then filter out the product, wash the product with water and alcohol three times successively; after washing, vacuum dry to obtain 2-hydroxy-3-sulfopropyl Cellulose ether, a sunflowe...

Embodiment 3

[0030] Use sunflower seed shells to wash, mash, dry, grind, and pass through a 70-mesh sieve, and use 8% HNO 3 Reflux for 3 hours, then reflux with 4% NaOH for 2 hours, wash with water and dry to obtain sunflower seed shell cellulose; take 20 g of the prepared cellulose and place it in a three-necked bottle, add 20 ml of NaOH solution with a concentration of 3 mo / L, 60 ml of Epichlorohydrin, heated to reflux for 2 hours, filtered; cross-washed with acetone and water until neutral, dried at 70°C to obtain light yellow cross-linked cellulose; pour 30g of the obtained cross-linked cellulose into a beaker, the beaker Put it in a water bath environment at 20°C, then add 20g of sodium bisulfite, 20g of sodium sulfite, and 100g of water into the beaker, and stir continuously with an electric stirrer. After reacting for 2 hours, add 1mol / L dioxane into the container Aqueous solution 100ml and 1mol / LNa 2 CO 3 100ml solution, reacted at 60°C for 1 hour, filtered out the product, washe...

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PUM

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Abstract

The invention discloses a preparation method of a sunflower flower seed husk adsorption material. The preparation method includes selecting sunflower flower seed husks to perform cleaning, mashing, drying, milling and sieving; performing acid and alkali heating reflux, washing and drying on sieved powder so that an initial product can be obtained; performing reaction and crosslinking on the initial product with a NaOH solution and epichlorohydrin; performing mixing reaction on crosslinked cellulose with 3-chloro-2-hydroxypropanesulfonic acid sodium salt, a dioxane aqueous solution and a Na2CO3solution; and performing intersecting washing on a product by successively using acetone and water so that a sunflower flower seed husk adsorption material finished product can be obtained after cleaning and vacuum drying. The adsorption material and preparation method are simple in process flow, low in cost, rich in raw material and friendly to environment.

Description

technical field [0001] The invention relates to a preparation method of an adsorption material, in particular to a preparation method of a sunflower seed shell adsorption material. Background technique [0002] With the development of electroplating, mining, chemical industry and other industries, heavy metal pollution is becoming more and more serious, and there are more and more pollution sources, such as mine drainage, waste rock field leaching water, ore dressing plant tailings drainage, non-ferrous metal smelting plant dust removal drainage, non-ferrous metal Pickling water in processing plants, washing water in electroplating plants, pickling water in iron and steel plants, and wastewater from industries such as electrolysis, pesticides, medicine, paints, and pigments are all important sources of heavy metal wastewater. Heavy metal pollution is different from other pollution sources. Other pollution sources can be automatically degraded through natural methods to reduc...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): B01J20/26B01J20/30C02F1/28C02F101/20
CPCB01J20/24B01J20/267C02F1/285C02F2101/20
Inventor 李海鱼
Owner 李海鱼