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A method for synchronously purifying arsenic ions and fluorine ions in industrial wastewater by stripping waste rocks from mining

A technology of industrial wastewater and fluorine ions, applied in the field of resources and environment, can solve the problems of complicated process and difficult fluorine discharge standards, and achieve the effects of simple process, low treatment cost and reduced risk of environmental pollution

Active Publication Date: 2021-09-03
KUNMING UNIV OF SCI & TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

The iron salt-lime step-by-step method of extracting arsenic and fluorine requires oxidizing trivalent arsenic to pentavalent arsenic first. The process is relatively complicated, and it is difficult for fluorine to meet the emission standard.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0026] Example 1: In this example, dolomite-type mining stripping waste rock is used to remove arsenic and fluoride ions in mineral processing wastewater.

[0027] The tailings wastewater produced by a lead-zinc beneficiation plant in Guangxi contains 0.30 mg / L arsenic and 3.3 mg / L fluorine, and the pH of the wastewater is neutral. Dolomite is used as an adsorbent to reduce the content of arsenic and fluorine in wastewater. After analysis, the main component of waste rock in the mining area is dolomite. The specific steps for removal are as follows:

[0028] (1) The waste rock is crushed and ground to a particle size of less than 1 mm by mass;

[0029] (2) Add 0.5mol / L KOH to 0.6mol / L FeCl 3 solution and mechanically stirred for 1h to mix evenly, wherein, KOH solution and FeCl 3 The volume ratio of the solution is 5:1, and then aged at 25°C for 2 days to prepare the hydroxyl iron pillar solution;

[0030] (3) Add the waste rock after crushing and grinding in step (1) to the...

Embodiment 2

[0034] Embodiment 2: In this embodiment, arsenic and fluoride ions in mineral processing wastewater are purified by using chlorite-type layered mining stripping waste rocks.

[0035] The waste rock stripped by a mining company in Yunnan mainly contains chlorite and a small amount of quartz. The wastewater generated on site is neutral, containing 0.62 mg / L and 4.2 mg / L of arsenic and fluorine respectively. The specific steps for removal are as follows:

[0036] (1) Ore crushing by crusher-grinding machine, and the particle size range of waste rock is controlled at -0.074mm~+0.037mm;

[0037] (2) Add 0.10mol / L NaOH to 0.2mol / L Al 2 (SO 4 ) 3 solution and stirred for 2h to mix evenly, among them, NaOH solution and Al 2 (SO 4 ) 3 The volume ratio of the solution is 2:1, and then aged at 23° C. for 1 day to prepare a hydroxyaluminum pillaring liquid;

[0038] (3) Add the waste rock after crushing and grinding in step (1) to the aged aluminum hydroxy propping solution in step...

Embodiment 3

[0042] Embodiment 3: In this embodiment, chlorite-type mining stripping waste rocks are used to purify the acidic arsenic-containing and fluorine-containing waste water produced in the mining area of ​​the mine.

[0043] A polymetallic mine in Hunan produced a large amount of acidic wastewater during the mining process, with a pH of 2 to 4, and the content of arsenic and fluorine in the solution was as high as 0.73mg / L and 5.4mg / L. In order to purify the water quality, the "neutralization-waste rock adsorption" process is adopted on site for treatment. The main components of the waste rock produced by the self-stripping process in the mining area are quartz and chlorite. The specific steps for removal are as follows:

[0044] (1) The waste rock is crushed and ground to a particle size of less than 2mm by mass;

[0045] (2) Add 1mol / L KOH to 1mol / L FeCl 3 solution and mechanically stirred for 4h to mix evenly, wherein, KOH solution and FeCl 3 The volume ratio of the solution...

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Abstract

The invention discloses a method for synchronously purifying arsenic ions and fluorine ions in industrial waste water from mining stripping waste rocks. Carry out modification, use the modified waste rock as an adsorbent, and adsorb arsenic ions and fluoride ions in industrial wastewater under the condition of pH 5-9 in the solution environment, and reduce the concentration of arsenic and fluoride ions in industrial wastewater. The invention uses modified mining stripping waste rock as a new adsorbent, which realizes the comprehensive utilization of solid waste, reduces the stockpiling of solid waste and the risk of environmental pollution, and reduces the purification cost of arsenic and fluorine ions in industrial wastewater The removal rate of the arsenic ion and the fluorine ion in the waste water can reach more than 95%. The method of the invention has the advantages of simple process, convenient operation, low treatment cost, environmental protection and good industrial application prospect.

Description

technical field [0001] The invention relates to a method for synchronously purifying arsenic ions and fluorine ions in industrial waste water from stripping waste rocks from mining, specifically a silicate mineral or carbonate mineral waste rock with a layered or pore structure produced by mining stripping, The invention relates to a method for adsorbing industrial waste water containing arsenic and fluorine after modification at normal temperature, belonging to the technical field of resources and environment. Background technique [0002] At present, arsenic in the natural environment is mainly composed of two parts, one is arsenic from rock minerals, and the arsenic in rocks will be gradually released into the surrounding environment under natural conditions; Arsenic wastewater. Most of the compounds of arsenic are poisonous and can cause skin diseases such as black foot disease, keratinization and even cancer. At present, the main removal methods of arsenic can be divi...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J20/16B01J20/30C02F1/28C02F101/14
CPCB01J20/0277B01J20/16C02F1/281C02F2101/14
Inventor 吕晋芳李秀全英聪童雄郑永兴
Owner KUNMING UNIV OF SCI & TECH