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A gas-solid fluidization method for preparing oxygen-free passivated titanium and titanium alloy powder products

A titanium alloy and powder technology, applied in the direction of gaseous chemical plating, additive manufacturing, metal processing equipment, etc., can solve the problems of large amount of coating on the surface of the powder, difficulty in achieving the coating effect, and difficult removal of sintering, etc. Uniform oxygen passivation layer, improved application environment and process, and easy control

Active Publication Date: 2021-06-11
UNIV OF SCI & TECH BEIJING
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, it is difficult to control the use of liquid organic matter coating. Too high solution concentration will lead to too much coating on the powder surface, which is difficult to remove after sintering, and too low solution concentration will make it difficult to achieve the coating effect

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0025] 30μm hydrodehydrogenation (HDH) pure titanium powder and VCl 4 The mass ratio is 80:20, and the concrete preparation steps are as follows:

[0026] (1) VCl meeting the formula requirements 4 and HDH pure titanium powder are respectively placed in the gasifier and the fluidized bed reactor;

[0027] (2) Heat the vaporizer to 180°C to make VCl 4 Vaporization, the VCl 4 Pass in the fluidized bed reactor together with dry argon according to volume ratio 20:80;

[0028] (3) Open the fluidized bed, and heat the fluidized bed to 300° C., feed the argon gas and metal halide gas to fluidize the titanium powder for 80 minutes, and obtain an oxygen-free passivated titanium powder after cooling;

[0029] (4) The oxygen-free passivated titanium powder obtained in step (3) is formed by an injection molding process using a polyoxymethylene-based binder system to obtain a green body;

[0030] (5) The green body obtained in step (4) is first deacidified at 120°C, then heated at 2°C...

Embodiment 2

[0032] 20μm gas atomized Ti-40Al titanium alloy powder and SnCl 4 The mass ratio is 92:8, and the whole operation and device are carried out under an argon protective atmosphere. Concrete preparation steps are as follows:

[0033] (1) SnCl that meets the formulation requirements 4 and Ti-40Al titanium powder are respectively placed in the gasifier and the fluidized bed reactor;

[0034] (2) Heat the vaporizer to 120°C to make SnCl 4 Gasification, the SnCl 4 Pass in the fluidized bed reactor together with dry argon according to volume ratio 15:85;

[0035] (3) Open the fluidized bed, and heat the fluidized bed to 150° C., feed the argon gas and metal halide gas to fluidize the titanium powder for 50 minutes, and obtain an oxygen-free passivated Ti-40Al titanium powder after cooling;

[0036] (4) The oxygen-free passivated titanium powder obtained in step (3) is pressed into shape using cold isostatic pressing;

[0037] (5) the green body obtained in the step (4) is placed...

Embodiment 3

[0039] -500 mesh ion spheroidized TC4 powder and SnCl 4 The mass ratio is 95:5, and the whole operation and device are carried out under an argon protective atmosphere. Concrete preparation steps are as follows:

[0040] (1) Metal halides and TC4 powder meeting the formula requirements are placed in the gasifier and the fluidized bed reactor respectively;

[0041] (2) Heat the vaporizer to 150°C to make SnCl 4 Gasification, the SnCl 4 Pass in the fluidized bed reactor together with dry argon according to volume ratio 10:90;

[0042](3) Open the fluidized bed, and heat the fluidized bed to 500° C., feed the argon gas and metal halide gas to fluidize the titanium powder for 30 minutes, and obtain an oxygen-free passivated titanium powder after cooling;

[0043] (4) The oxygen-free passivated titanium powder obtained in step (3) is carried out by gel injection molding using a low molecular weight gel system;

[0044] (5) Heat the green body obtained in step (4) in argon at 2...

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Abstract

A method for preparing oxygen-free passivated titanium and titanium alloy powder products by gas-solid fluidization belongs to the field of powder metallurgy titanium. The present invention proposes to realize gas-solid fluidization of low-boiling metal halides through a fluidized bed, to react metal halides with titanium powder, and uniformly deposit a layer of oxygen-free passivation layer with controllable thickness and uniform thickness on the surface of titanium powder. Effectively achieve low gap control of titanium powder; at the same time, gaseous TiX x o y The formation of titanium powder is conducive to breaking the oxide film on the surface of titanium powder, purifying the surface of titanium powder particles, and promoting sintering densification, and metal alloy elements are conducive to further sintering densification or microalloying of titanium products, thereby improving the comprehensive performance of titanium products. The present invention uses fluidized bed gas-solid fluidization to prevent uneven passivation caused by agglomeration and adhesion of powder, has no restrictions on particle size distribution, shape and type of titanium powder, is widely used and simple in process, and can be continuously operated in large quantities .

Description

technical field [0001] The invention belongs to the field of titanium powder metallurgy and provides a method for realizing oxygen-free passivation of titanium and titanium alloy powder by gas-solid fluidization. Background technique [0002] Powder metallurgy titanium and titanium alloys have uniform structure, fine grains, and near-net shape characteristics, which have attracted widespread attention of titanium workers around the world. However, due to the large specific surface area of ​​the powder, especially titanium and titanium alloy powders with finer particle sizes, they are extremely sensitive to interstitial elements such as oxygen, nitrogen, and hydrogen. Impurity elements such as oxygen and nitrogen are easily adsorbed on the surface of titanium powder, resulting in the impurity content of titanium powder Increase. On the one hand, the oxygen (O) content of interstitial atoms is one of the key factors affecting the mechanical properties of titanium, and the che...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B22F9/30B22F1/145B22F1/16
CPCB22F9/30B22F2202/15B22F2998/10B22F2999/00B22F1/145B22F1/16B22F3/04B22F3/1007B22F3/22B22F2201/20B22F9/023B22F3/225B22F3/1021B22F9/082B22F3/1017B22F3/02B22F1/107B33Y10/00B33Y70/00B33Y80/00B22F10/14Y02P10/25C23C16/442C23C16/4417C23C16/4488C23C16/08B22F3/16B22F2301/205C23C16/4481
Inventor 杨芳邵艳茹周洋郭志猛隋延力秦乾陈存广
Owner UNIV OF SCI & TECH BEIJING