Optical film adhesive, adhesive layer, optical member, and image display apparatus
A technology for optical components and optical films, applied in adhesive types, ester copolymer adhesives, adhesives, etc., can solve problems such as durability test shrinkage
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preparation example 1
[0299] [Preparation Example 1: Preparation of a solution of (meth)acrylate copolymer (A1)]
[0300] Into a four-necked flask equipped with a stirring blade, a thermometer, a nitrogen inlet pipe and a cooler, 50 parts by weight of n-butyl acrylate (Nippon Shokubai Co., Ltd.), 29 parts by weight of 2-ethylhexyl acrylate (Osaka Organic Chemical Industry Co., Ltd.), 10 parts by weight of methyl acrylate (Nippon Shokubai Co., Ltd.) and 2-ethylhexyl diglycol acrylate (Kyoeisha Chemical Co., Ltd.), 1 part by weight of acrylic acid 4 - Hydroxybutyl ester (Osaka Organic Chemical Industry Co., Ltd.) and 0.1 parts by weight of 2,2'-azobisisobutyronitrile (Wako Junyaku Kogyo Co., Ltd.) as a polymerization initiator and 100 parts by weight of acetic acid Ethyl ester, then gently stir the components while introducing nitrogen into the flask. After purging with nitrogen, the temperature of the liquid in the flask was raised to reflux of ethyl acetate, followed by polymerization for 5 hours ...
preparation example 1 to 15
[0301] [Preparation Examples 1 to 15: Preparation of Solutions of (Meth)acrylate Copolymers (A2) to (A15)]
[0302] (Meth)acrylic acid was prepared in the same manner as in Preparation Example 1, except that the monomer types and mixing ratios of each (meth)acrylate were changed as listed in Table 1 and the amount of polymerization initiator and reaction time were appropriately changed. Solutions of Ester Copolymers (A2) to (A15). Table 1 shows the measurement results of glass transition temperature (Tg), weight average molecular weight (Mw) and dispersion index (Mw / Mn) of each (meth)acrylate copolymer (A2) to (A15). In Table 1, a blank indicates that no monomer was used.
[0303] Table 1
[0304]
[0305] Note) BA: n-butyl acrylate (Nippon Shokubai Co., Ltd., Tg in homopolymer phase: -45°C)
[0306] 2EHA: 2-ethylhexyl acrylate (Nippon Shokubai Co., Ltd., Tg in homopolymer phase: -68°C)
[0307] MEA: 2-methoxyethyl acrylate (Nippon Shokubai Co., Ltd., Tg in homopolymer ...
Embodiment 1
[0315] [Preparation of adhesives for optical films]
[0316] While stirring, 100 parts by weight of the solid (meth)acrylate copolymer A1 solution obtained in Preparation Example 1 (ie 100 parts by weight of (meth)acrylate (A1)) and 0.1 parts by weight as a crosslinking agent B's D-110N (75% ethyl acetate solution of trimethylolpropane adduct of xylene diisocyanate) (Mitsui Kagaku Co., Ltd., number of isocyanate groups per molecule: 3) and 0.1 parts by weight as silane KBM-403 (3-glycidoxypropyltrimethoxysilane) (Shin-Etsu Kagaku Kogyo Co., Ltd.) of the coupling agent (C) was mixed, thereby preparing an adhesive for an optical film (Solid content: 25% by weight).
[0317] [Formation of adhesive layer]
[0318] The obtained adhesive for optical films was coated onto a 38 μm thick silicone-treated polyethylene terephthalate (PET) film (MRF38, Mitsubishi Chemical Co., Ltd., oligomer-free on one surface of the object prevention layer) so that the adhesive layer has a thicknes...
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