Application of phenazine-1-carboxamide modified compound 18-3 in inhibition of strawberry gray mould
A technology of botrytis cinerea and formamide, applied in the application, fungicide, organic chemistry and other directions, can solve the problem of weak bacteriostatic effect, etc., and achieve the effect of strong inhibition effect, good inhibition effect and difficult drug resistance
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Embodiment 1
[0014] Example 1 Preparation of phenazine-1-carboxamide modified compound 18-3
[0015] The synthetic method of modified compound 18-3: hydrolyze phenazine-1-carboxamide under acidic conditions to generate phenazine-1-carboxylic acid; take 6.2 mmol phenazine-1-carboxylic acid (1.4179 g), 6.2 mmol 4- Phenylbutylamine (1ml), 12.4mmol tris(trifluoroethoxy)boron (2.675ml), and 12.4ml acetonitrile were added to a 25ml round-bottomed flask, stirred magnetically, and reacted at 80°C for 24h; after the reaction solution was cooled, 20ml of DCM and 3 ml of water; then add 930 mg of Amberlyst A-26 (OH), Amberlyst 15, and AmberliteIRA743 resin in turn, and stir at room temperature for 30 min; then add anhydrous magnesium sulfate powder to remove water, filter, and use dry DCM to wash solid magnesium sulfate 3 times, Rotary evaporation to obtain the modified product 18-3 with a yield of 52.64%.
Embodiment 2
[0016] Example 2 Structure identification of phenazine-1-carboxamide modified compound 18-3
[0017] By hydrogen spectrum (1H NMR (500MHz, CDCl3) δ11.04 (s, 54H), 9.05–8.86 (m, 56H), 8.52–7.66 (m, 363H), 7.29 (s, 10H), 7.33–7.14 (m ,15H),4.03–3.44(m,255H),3.41(d,J=3.3Hz,163H),3.35(t,J=4.6Hz,13H),2.67(s,4H),2.33(d,J= 13.9Hz, 4H), 2.18–2.01 (m, 122H), 1.83 (dd, J=12.6, 6.1Hz, 4H), 1.48–1.14 (m, 107H), 1.74–0.78 (m, 275H), 1.53–0.78 (m, 253H), 1.00 (ddd, J=18.6, 14.5, 7.3Hz, 26H), 0.93–0.50 (m, 119H), -0.00 (s, 14H).), carbon spectrum (13C NMR (126MHz, CDCl3) )δ164.77(s), 143.41(s), 142.91(s), 141.33(s), 140.84(s), 135.35(s), 133.52(s), 131.60(s), 131.00(s), 130.09( s), 129.69(s), 129.21(s), 129.02(s), 77.32(s), 77.07(s), 76.81(s), 70.94(s), 58.80(s), 37.46(s), 29.52( s).) and mass spectrum (molecular weight: 295.20, figure 1 ) The compound synthesized by detection example 1 is consistent with the expected target, and its molecular formula is C 23 H 21 N 3 O, the structura...
Embodiment 3
[0020] (1) Instruments and related materials
[0021] YJ-VS-2 ultra-clean workbench (Wuxi Yijing Purification Equipment Co., Ltd.), LDZX-30E sterilizer (Shanghai Shen'an Medical Equipment Factory), MPJ-250 incubator (Shanghai Senxin Experimental Instrument Co., Ltd.) , QHX-400B-III type light incubator (Shanghai Xinmiao Medical Equipment Manufacturing Co., Ltd.), electric furnace (Beijing Zhongxing Weiye Instrument Co., Ltd.), etc., as well as measuring cylinders, glass rods, beakers, triangular flasks, rulers, pencils, label paper, Parafilm, picking needle, volumetric flask, inoculation needle, ph-101 watering can, hole punch, petri dish, kitchen knife, gauze.
[0022] ⑵ medicine
[0023] The original drug of 93% phenazine-1-carboxamide modified product 18-3 (hereinafter referred to as modified product 18-3) prepared in Example 1; agar, glucose, acetone and Tween 80 were purchased from Sinopharm Group.
[0024] (3) strain
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