Preparation method of silicon carbide crystal, silicon carbide wafer, silicon carbide substrate and semiconductor device
A silicon carbide single crystal and silicon carbide technology is applied in the preparation of silicon carbide crystals, silicon carbide substrates and semiconductor devices, and silicon carbide wafers. Silicon crystal quality and other issues, to achieve the effect of reducing reaction temperature, improving quality and reducing process cost
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[0034] In order to improve the quality of silicon carbide crystals prepared by HTCVD, the present invention proposes a method for preparing silicon carbide crystals, and the figure shows an example of the method for preparing silicon carbide crystals provided by the present invention. refer to figure 1 As shown, in this embodiment, the preparation method of the silicon carbide crystal comprises the following steps:
[0035] Step S10, methyltrichlorosilane (CH 3 Cl 3 Si) and hydrogen (H 2 ) Reductive decomposition reaction is carried out in the first reaction chamber to generate silicon tetrahydride and ethane;
[0036] Use CH 3 Cl 3 Si is the raw material, and H 2 A reduction decomposition reaction occurs, and its reaction equation is as follows:
[0037] 2CH 3 Cl 3 Si+7H2→2SiH 4 ↑+6HCl↑+C 2 h 6 ↑
[0038] In the reductive decomposition reaction, CH 3 Cl 3 Si is the raw material, and H 2The reaction produces gas SiH 4 , HCl and C 2 h 6 , due to CH 3 Cl 3 S...
Embodiment 1
[0068] (1) to CH 3 Cl 3 Si is used as a raw material for dry passivation to remove the water vapor, and then the CH 3 Cl 3 Si and H 2 According to the molar ratio of 2:7, it is passed into the first reaction chamber, and the reduction and decomposition reaction is carried out under the conditions of 1000 ° C and 1.2 Pa to generate SiH 4 , HCl and C 2 h 6 ;
[0069] (2) SiH generated in step (1) 4 and C 2 h 6 (SiH 4 and C 2 h 6 The molar ratio is 2:1) into the second reaction chamber, and the reaction is carried out at 1550°C and 0.6Pa to generate SiC and H 2 ;
[0070] (3) The SiC generated in step (2) is in contact with the seed crystal set in the second reaction chamber, and under the conditions of 1550°C and 0.3Pa, it nucleates and grows at the seed crystal, and crystallizes to form silicon carbide single crystals and grow into silicon carbide crystals.
Embodiment 2
[0072] (1) to CH 3 Cl 3 Si is used as a raw material for dry passivation to remove the water vapor, and then the CH 3 Cl 3 Si and H 2 According to the molar ratio of 2:7, it is passed into the first reaction chamber, and the reduction and decomposition reaction is carried out under the conditions of 1100 ° C and 1.1 Pa to generate SiH4 , HCl and C 2 h 6 ;
[0073] (2) SiH generated in step (1) 4 and C 2 h 6 (SiH 4 and C 2 h 6 The molar ratio is 2:1) into the second reaction chamber, and the reaction is carried out at 1600°C and 0.5Pa to generate SiC and H 2 ;
[0074] (3) The SiC generated in step (2) is in contact with the seed crystal set in the second reaction chamber, and under the conditions of 1600°C and 0.5Pa, it nucleates and grows at the seed crystal, and crystallizes to form silicon carbide single crystals and grow into silicon carbide crystals.
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