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Manufacturing method of flexible lithium metal battery negative electrode

A technology for lithium metal batteries and manufacturing methods, which is applied to battery electrodes, lithium storage batteries, active material electrodes, etc., can solve problems such as inability to achieve uniform deposition of lithium metal, low Coulombic efficiency, and insufficient lithium affinity, and achieve excellent cycle performance, High Coulombic efficiency and light weight effect

Active Publication Date: 2022-05-27
WANXIANG 123 CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0006] The present invention is to overcome the problem that the negative electrode of the existing lithium metal battery adopts a metal matrix, the density of the metal material is high, resulting in low energy density and insufficient flexibility; the use of conductive carbon material, insufficient lithium affinity can not realize the uniform deposition of lithium metal, resulting in low coulombic efficiency Insufficient, to provide a flexible lithium metal negative electrode manufacturing method with small mass, high energy density, high Coulombic efficiency, and excellent cycle performance

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0033] A. Wash the absorbent cotton cloth in deionized water and dry it;

[0034] B. The absorbent cotton cloth obtained in step A is immersed in an aqueous solution of 10wt% EDTA disodium copper solution, soaked for 1 hour and taken out, and dried at 60°C in a constant temperature blast oven;

[0035] C. The sample obtained in step B was placed in a porcelain ark, carbonized in a tube furnace under nitrogen atmosphere, the carbonization process was raised to 280 °C at a heating rate of 3 °C / min, and kept for 4 h; then, at a temperature of 7 °C / min The heating rate was raised to 900 °C, and the temperature was kept for 2 h; the heating was stopped and allowed to cool to room temperature naturally to obtain a carbon fiber cloth with carbon-supported metal particles;

[0036] D. immerse the carbon fiber cloth of the carbon-loaded metal particles obtained in step C in the ethanol solution of 2-methylimidazole whose mass fraction is 3wt%, take out after soaking for 24 hours, and d...

Embodiment 2

[0040] A. Wash the absorbent cotton cloth in deionized water and dry it;

[0041] B. The absorbent cotton cloth obtained in step A is immersed in an aqueous solution of 15wt% EDTA disodium copper solution, soaked for 6 hours and taken out, and dried at 60°C in a constant temperature blast oven;

[0042] C. The sample obtained in step B was placed in a porcelain ark, carbonized in a tube furnace under nitrogen atmosphere, the carbonization process was raised to 260 °C at a heating rate of 3 °C / min, and kept for 3 hours; then, at a temperature of 7 °C / min The heating rate was raised to 700°C, and the temperature was kept for 4 hours; the heating was stopped and allowed to cool to room temperature naturally to obtain carbon fiber cloth with carbon-supported metal particles;

[0043] D. immerse the carbon fiber cloth of the carbon-loaded metal particles obtained in step C in the ethanol solution of 2-methylimidazole with a mass fraction of 1 wt%, take out after soaking for 48 hour...

Embodiment 3

[0047] A. Wash the absorbent cotton cloth in deionized water and dry it;

[0048] B. The absorbent cotton cloth obtained in step A is immersed in a mixed aqueous solution of 15wt% EDTA disodium nickel and 10wt% EDTA disodium copper mixed solution, soaked for 6 hours and taken out, and dried at 60°C in a constant temperature blast oven;

[0049] C. The sample obtained in step B was placed in a porcelain ark, carbonized in a tube furnace under nitrogen atmosphere, the carbonization process was raised to 270 °C at a heating rate of 3 °C / min, and kept for 2 hours; then, at a temperature of 7 °C / min The heating rate was raised to 800°C, and the temperature was kept for 3 hours; the heating was stopped and allowed to cool to room temperature naturally to obtain a carbon fiber cloth with carbon-supported metal particles;

[0050] D. immerse the carbon fiber cloth of the carbon-loaded metal particles obtained in step C in a melamine acetic acid solution whose mass fraction is 5wt%, ta...

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Abstract

The invention relates to the field of lithium metal batteries, and aims to overcome the defects of low energy density and insufficient flexibility caused by high density of a metal material due to adoption of a metal matrix in an existing negative current collector; in order to overcome the defect of low coulombic efficiency caused by incapability of realizing uniform deposition of lithium metal due to small specific surface area due to use of a carbon fiber material, the invention discloses a manufacturing method of a flexible lithium metal battery negative electrode. Metal ions are attached in organic fiber cloth and calcined, then nitrogen-doped modified calcination is carried out, carbon fiber cloth of nitrogen-doped carbon loaded metal particles is obtained, then lithium metal is loaded, and the flexible lithium metal battery negative electrode is obtained. The obtained lithium metal battery negative electrode has the advantages of good flexibility, light weight, high energy density, large specific surface area, high coulombic efficiency, high safety performance and excellent cycle performance.

Description

technical field [0001] The invention relates to the field of lithium metal batteries, in particular to a method for manufacturing a negative electrode of a flexible lithium metal battery. Background technique [0002] With the development of society, people's demand for the battery life of electronic devices is getting higher and higher, and traditional lithium-ion batteries can no longer meet the needs of battery development. Compared with the existing graphite anodes and even higher capacity silicon-oxygen and silicon-carbon material anodes, metal lithium has a low electrochemical potential (-3.045V)) and a high theoretical capacity (3860mA·h·g) -1 ), low density (0.534g cm -3 ), which makes lithium metal batteries have high energy density and is the most potential lithium secondary battery material. However, due to its high electrochemical reactivity and no host characteristics, metal lithium anode usually brings two major problems of safety and cycle life. The lithium ...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): H01M4/66H01M4/70H01M4/134H01M4/1395H01M10/052
CPCH01M4/667H01M4/70H01M4/134H01M4/1395H01M10/052H01M2004/027Y02E60/10
Inventor 陆佳婷郭彬林王慧敏韩笑李凡群
Owner WANXIANG 123 CO LTD