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Inorganic combustion inhibitor of polyphosphoric acid radical column supported hydrotalcite and method for preparing same

A technology of polyphosphate column and inorganic flame retardant, which is applied in the direction of fire retardant coatings, can solve the problems of deterioration of physical and mechanical properties of materials, difficulty in material processing, etc., to improve compatibility and dispersibility, less equipment investment, and source of raw materials. wide effect

Inactive Publication Date: 2011-10-05
ZHEJIANG UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Although hydrotalcite has the functions of flame retardancy, smoke elimination and filling enhancement, it will deteriorate the physical and mechanical properties of the material and bring many difficulties in material processing

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0020] 1) Calcining the commercially available magnesium-aluminum hydrotalcite at 450°C for 1 hour, grinding it to less than 200 mesh, and the obtained product is a bimetallic oxide;

[0021] 2) Weigh 94.2 grams of potassium acetate, add water to prepare an aqueous solution with a concentration of 1.5 mol / L, then add 188.4 grams of bimetallic oxide, stir in a water bath at 40°C for 2 hours, filter, wash with water, and dry to obtain acetate intercalation water Talc pillared precursors;

[0022] 3) Weigh 100 grams of the acetate intercalated hydrotalcite pillar precursor obtained in step 2), add 20 grams of ammonium polyphosphate with a degree of polymerization of 10, mix, add a small amount of water to grind for 10 minutes, place in a water bath at 40°C for 2 hours, and filter , washed with water, and dried to obtain the product polyphosphate pillared hydrotalcite.

[0023] 4) Take the polyphosphate pillared hydrotalcite obtained in step 3), fully mix it according to the mass...

Embodiment 2

[0025] 1) Calcining the commercially available magnesium-aluminum hydrotalcite at 750°C for 5 hours, grinding it to less than 200 mesh, and the obtained product is a bimetallic oxide;

[0026] 2) Weigh 82.03 grams of sodium acetate, add water to prepare an aqueous solution with a concentration of 2 mol / L, then add 410.15 grams of bimetallic oxide, stir for 5 hours in a water bath at 80°C, filter and wash with water, and dry at a temperature of 90°C to obtain Acetate intercalated hydrotalcite pillar precursor;

[0027] 3) Weigh 100 grams of the acetate intercalated hydrotalcite pillar precursor obtained in step 2), add 80 grams of ammonium polyphosphate with a degree of polymerization of 20, mix, add a small amount of water to grind for 20 minutes, place in a water bath at 80°C for 5 hours, and filter , washed with water, and dried at 90°C to obtain the product polyphosphate pillared hydrotalcite.

[0028] 4) Take the polyphosphate pillared hydrotalcite obtained in step 3), fu...

Embodiment 3

[0030] 1) Calcining the commercially available magnesium-aluminum hydrotalcite at 500°C for 4 hours, grinding it to less than 200 mesh, and the obtained product is a bimetallic oxide;

[0031] 2) Weigh 77.08 grams of ammonium acetate, add water to prepare an aqueous solution with a concentration of 1.5 mol / L, then add 308.32 grams of double metal oxide, stir in a water bath at 60°C for 4 hours, filter, wash with water, and dry to obtain acetate intercalation water Talc pillared precursors;

[0032] 3) Weigh 100 grams of the acetate intercalated hydrotalcite pillar precursor obtained in step 2), add 30 grams of ammonium polyphosphate with a degree of polymerization of 15, mix, add a small amount of water to grind for 15 minutes, place in a water bath at 60°C for 4 hours, and filter , washed with water, and spray-dried to obtain the product polyphosphate pillared hydrotalcite.

[0033]4) Take 100 parts of PVC resin, 60 parts of dibutyl phthalate, 15 parts of titanium dioxide, 1...

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Abstract

The invention discloses a polyphosphoric acid radical pillared hydrotalcite inorganic flame retardant and a method for making the same. The method is to calcine hydrotalcite as raw material to obtain bimetal oxides, hydrate the bimetal oxides in an acetate solution to obtain an acetate intercalation hydrotalcite pillared precursor, grind the pillared precursor together with oligomeric phosphate after drying the pillared precursor, and obtain polyphosphoric acid radical pillared hydrotalcite through secondary intercalation. On the basis of keeping the layered structure of hydrotalcite, a product is combined with the polymer structure of oligomeric phosphate, overcomes the disadvantage that oligomeric ammonium phosphate is difficult to be used as flame retardant of plastics because of low melting point and sintering point, simultaneously improves the compatibility with polymer as well as dispersity, and has multiple efficacy of retarding flame, filling, plasticizing, enhancing, suppressing smoke, etc. The method for making polyphosphoric acid radical pillared hydrotalcite is simple, little in equipment investment and extensive in raw material source. Moreover, the raw material, the product and the thermal decomposition product thereof are all nontoxic and harmless.

Description

technical field [0001] The invention relates to a polyphosphate root pillared hydrotalcite inorganic flame retardant and a preparation method thereof. Background technique [0002] Synthetic polymer materials are widely used in various fields such as building materials, electronic appliances, daily furniture, interior decoration, transportation, etc., and play a huge role in national economic construction and people's lives. However, a considerable part of the fires that have occurred in recent years are caused by the ignition of polymer materials. With the development of synthetic materials industry and the continuous expansion of application fields, flame retardants have broad development prospects; in addition, fields such as coal fields, oil fields, and forest fires have also promoted the rapid development of flame retardants and fire extinguishing agents in my country. It has developed into the second largest polymer material modification additive after plasticizers. ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C09K21/04
Inventor 叶瑛夏枚生李秀悌姚志通邬黛黛陈雪刚韩沉花胡秀芳
Owner ZHEJIANG UNIV