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Method for recycling aniline and methanol from mixed waste water of aniline and methanol

A technology of mixing wastewater and methanol water, which is applied in chemical instruments and methods, preparation of organic compounds, preparation of hydroxyl compounds, etc., can solve the problems of wasting resources and increasing the difficulty of treatment, and achieve the effect of high recovery efficiency and simple process

Active Publication Date: 2013-11-27
JINAN SHENGQUAN GROUP SHARE HLDG
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0003] In the existing chemical production, there is often mixed wastewater containing aniline and methanol, which is often directly sent to the sewage treatment plant for treatment without recycling. This increases the difficulty of treatment on the one hand, and wastes resources on the other hand.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0017] Take 1000g of mixed wastewater containing aniline and methanol (aniline content 20%, methanol content 30%), concentrate under reduced pressure at 50 degrees vacuum -0.09Mpa to 250g (methanol content is less than 1%), cool down to 25 degrees, and stand layered. The lower layer is the aniline layer, and 180 g of aniline is concentrated under reduced pressure at 80 degrees vacuum to -0.95 Mpa. The purity of aniline is greater than 98%, and the water content is less than 0.5%.

[0018] The upper layer is the water layer, which contains a small amount of methanol and aniline, and is extracted twice by adding 2*50g of dichloromethane. The methylene chloride layer was desolvated under reduced pressure at 40°C, and the remaining aniline was distilled under reduced pressure at 100°C to recover 15 g of aniline with a purity greater than 98%. The content of aniline in the upper water layer is less than 200 mg per liter, which can be treated by biochemical methods.

[0019] The d...

Embodiment 2

[0021] Take 1000g of mixed wastewater containing aniline and methanol (aniline content 35%, methanol content 15%), concentrate under reduced pressure to 400g (methanol content is less than 1%) under 70 degree vacuum degree-0.085Mpa, cool to 30 degrees, static Set layers. The lower layer is the aniline layer, and 300 g of aniline is concentrated under reduced pressure at 150 degrees vacuum degree-0.08Mpa. The purity of aniline is greater than 98%, and the water content is less than 0.5%.

[0022] The upper layer is the water layer, which contains a small amount of methanol and aniline, and is extracted twice by adding 2*50g of dichloromethane. The dichloromethane layer was desolvated under reduced pressure at 40°C, and the remaining aniline was distilled under reduced pressure at 100°C to recover 20 g of aniline with a purity greater than 98%. The content of aniline in the upper water layer is less than 200 mg per liter, which can be treated by biochemical methods.

[0023] T...

Embodiment 3

[0025] Take 1000g of mixed wastewater containing aniline and methanol (aniline content 15%, methanol content 35%), concentrate under reduced pressure at 60 degrees vacuum -0.08Mpa to 200g (methanol content is less than 1%), cool down to 30 degrees, and stand layered. The lower layer is the aniline layer, and 120 g of aniline is concentrated under reduced pressure at 100 degrees vacuum degree-0.09Mpa. The purity of aniline is greater than 98%, and the water content is less than 0.5%.

[0026] The upper layer is the water layer, which contains a small amount of methanol and aniline, and is extracted twice by adding 2*50g of dichloromethane. The dichloromethane layer was desolvated under reduced pressure at 40°C, and the remaining aniline was distilled under reduced pressure at 100°C to recover 15 g of aniline with a purity greater than 98%. The content of aniline in the upper water layer is less than 200 mg per liter, which can be treated by biochemical methods.

[0027] The d...

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Abstract

The invention provides a safe, reliable and efficient method for recycling aniline and methanol from mixed waste water of aniline and methanol. The method comprises the following steps of: utilizing a method for decompressing and distilling to distill methanol and parts of water from a mixed solvent; distilling until the methanol content is less than 1 and statically standing residual aniline and water to be layered, wherein the lower layer is the aniline layer; and evaporating the separated aniline layer through decompressing and distilling; adding dichloromethane into the water layer to extract the aniline, wherein the content of the residual water and aniline is very low and the residual water and aniline can be treated by utilizing a biochemical method; passing the distilled mixed solution of methanol and water through a rectifying tower to recycle the methanol. The method provided by the invention not only recycles aniline and methanol from the waste water but also solves the problem that the aniline-containing waste water is difficult to be treated.

Description

technical field [0001] The invention relates to a wastewater treatment and recovery method, in particular to a method for recovering aniline and methanol from mixed wastewater of aniline and methanol. Background technique [0002] Aniline is the simplest primary aromatic amine, a compound formed by replacing one of the hydrogen atoms in the benzene molecule with an amino group. It is a colorless oily flammable liquid with a strong odor. Melting point is -6.3°C, boiling point is 184°C, relative density is 1.0217 (20 / 4°C), refractive index is 1.5863, flash point (open cup) is 70°C, spontaneous ignition point is 770°C, decomposes when heated to 370°C, slightly soluble in water, easily Soluble in ethanol, ether, chloroform and other organic solvents. Turns brown when exposed to air or sunlight. It can be distilled with steam, and a small amount of zinc powder is added during distillation to prevent oxidation. 10-15ppm of NaBH4 can be added to the purified aniline to prevent o...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C07C31/04C07C29/80C07C211/46C07C209/86
Inventor 唐一林郗尊波高绍丰王锡龙
Owner JINAN SHENGQUAN GROUP SHARE HLDG