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Method for synthesizing rare earth Er-doped CdTe:Er quantum dot by hydrothermal method

A technology of quantum dots and hydrothermal method, applied in chemical instruments and methods, nanotechnology for materials and surface science, nanotechnology, etc., can solve the problem of poor fluorescence stability of CdTe quantum dots, high toxicity and volatile nature of CdTe quantum dots No foul odor and other problems, to achieve the effect of adjustable fluorescence emission wavelength, low cost, simple and convenient operation

Inactive Publication Date: 2014-03-12
GUANGXI TEACHERS EDUCATION UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

At present, the preparation of CdTe quantum dots mainly uses small molecules such as thioglycolic acid and mercaptopropionic acid as modifiers. Such small molecules are unstable and easily volatile, making the fluorescence stability of CdTe quantum dots poor and biocompatible. poor sex
In addition, the presence of heavy metal element Cd makes CdTe quantum dots more toxic, which limits its application in biochemical analysis and biomedicine.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0019] A kind of hydrothermal synthesis rare earth Er doped CdTe: the method of Er quantum dot, its step is as follows:

[0020] 1. Preparation of sodium telluride hydride NaHTe solution:

[0021] Put 0.2mmol tellurium powder and 0.4mmol sodium borohydride into a two-necked flask, add 5mL distilled water, protect with nitrogen, stir and react at 70°C for 60min to obtain sodium telluride hydride NaHTe solution for later use;

[0022] 2. Preparation of rare earth Er-doped CdTe:Er quantum dots

[0023] 0.02mmol CdCl 2 , 0.001 mmol Er 2 o 3 Dissolve 0.02mmol N-acetyl-L-cysteine ​​in 40mL distilled water, adjust the pH value to 7.0 with 1mol / L NaOH solution, blow nitrogen to remove oxygen, add 50mL sodium telluride hydride NaHTe solution prepared in step 1, and mix well Afterwards, it was transferred to a hydrothermal reaction kettle and heated to 180° C. to react for 60 minutes to obtain 40 mL of rare earth Er-doped CdTe:Er quantum dot solution with adjustable fluorescence emi...

Embodiment 2

[0025] A kind of hydrothermal synthesis rare earth Er doped CdTe: the method of Er quantum dot, its step is as follows:

[0026] 1. Preparation of sodium telluride hydride NaHTe solution

[0027] Put 0.4mmol tellurium powder and 1.2mmol sodium borohydride into a two-necked flask, add 4mL distilled water, protect with nitrogen, stir and react at 90°C for 30min to obtain sodium telluride hydride NaHTe solution for later use;

[0028] 2. Preparation of rare earth Er-doped CdTe:Er quantum dots

[0029] 0.4mmol CdBr 2 , 0.06mmol Er 2 o 3 Dissolve 0.8mmol N-acetyl-L-cysteine ​​in 20mL distilled water, adjust the pH value to 8.0 with 1mol / L NaOH solution, blow nitrogen to remove oxygen, add 2mL sodium telluride hydride NaHTe solution prepared in step 1, mix well Afterwards, it was transferred to a hydrothermal reaction kettle and heated to 190° C. for 30 minutes to obtain 22 mL of rare earth Er-doped CdTe:Er quantum dot solution with adjustable fluorescence emission wavelength an...

Embodiment 3

[0031] A kind of hydrothermal synthesis rare earth Er doped CdTe: the method of Er quantum dot, its step is as follows:

[0032] 1. Preparation of sodium telluride hydride NaHTe solution

[0033] Put 1.12mmol tellurium powder and 5.60mmol sodium borohydride into a two-necked flask, add 8mL distilled water, protect with nitrogen, stir and react at 100°C for 10min, and obtain sodium telluride hydride NaHTe solution for later use;

[0034] 2. Preparation of rare earth Er-doped CdTe:Er quantum dots

[0035] 1.4mmol CdI 2 , 0.56 mmol Er 2 o 3 Dissolve 4.2mmol of N-acetyl-L-cysteine ​​in 70mL of distilled water, adjust the pH value to 10.0 with 1mol / L NaOH solution, blow nitrogen to remove oxygen, add 8mL of sodium telluride hydride NaHTe solution prepared in step 1, and mix well Afterwards, it was transferred to a hydrothermal reaction kettle and heated to 200° C. for 5 minutes to obtain 78 mL of rare earth Er-doped CdTe:Er quantum dot solution with adjustable fluorescence emis...

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Abstract

The invention discloses a method for synthesizing a rare earth Er-doped CdTe:Er quantum dot by a hydrothermal method. The preparation method comprises the following operation steps: injecting a previously prepared NaHTe solution in a previously prepared mixed solution of cadmium salt, erbium oxide and water-soluble N-acetyl-L-cysteine under nitrogen protection to obtain a rare earth Er-mixed CdTe precursor solution, then putting the precursor solution in a hydrothermal reaction kettle for reaction to prepare the rare earth Er-doped CdTe:Er quantum dot with adjustable fluorescence emission wavelength and high fluorescence quantum yield. The method is carried out in a water solution and has the advantages that the raw materials are easy to acquire, the cost is low, the convenient and safe operation is realized, the environmental protection is realized and the like. The prepared rare earth Er-doped CdTe:Er quantum dot has the advantages of excellent fluorescence performance and great biologic compatibility and can be widely used in the fields of biochemical analysis and biomedicine as a novel fluorescent nanometer probe.

Description

technical field [0001] The invention belongs to the technical field of biochemical analysis and detection technology and nanometer material preparation, and specifically relates to a method for synthesizing CdTe:Er quantum dots doped with rare earth Er by a hydrothermal method. Background technique [0002] Quantum dots are inorganic semiconductor fluorescent nanocrystals composed of II-VI or III-V elements. Compared with traditional organic dyes, quantum dots have quite superior fluorescence properties, such as wide and continuous excitation spectrum, narrow and symmetrical emission spectrum, adjustable fluorescence emission wavelength, single excitation and multiple emission, high fluorescence stability, and photobleaching resistance. Strong, etc., making it play a huge role in the fields of biochemical analysis and biomedicine. Therefore, the synthesis of high-performance fluorescent nano-quantum dots has gradually attracted great attention. So far, quantum dots prepare...

Claims

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Application Information

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IPC IPC(8): C09K11/88B82Y20/00B82Y30/00B82Y40/00
Inventor 黄珊肖琦苏炜盛家荣彭炳华朱发伟
Owner GUANGXI TEACHERS EDUCATION UNIV