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A kind of preparation method of anode material of sodium ion battery

A sodium-ion battery and positive electrode material technology, which is applied in the field of electrochemistry, can solve the problems of low initial efficiency and poor cycle performance, and achieve the effects of high initial efficiency, good molding, and uniform coating

Inactive Publication Date: 2015-09-30
QILU UNIV OF TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] Aiming at the first low efficiency of sodium ion batteries in the prior art, the defects of poor cycle performance, one of the purposes of the present invention is to provide a kind of positive electrode material of sodium ion batteries, the composition of described material is Na 0.44 MnO 2 Conductive polymer, the material has good cycle and rate performance

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0022] (1) Add 0.23g (NH 4 ) 2 S 2 o 8 , 0.17g MnSO 4 ·H 2 O, 0.07g Na 2 SO 4 Add to 20g deionized water to make a uniform salt solution;

[0023] (2) Transfer the salt solution obtained in step (1) to a 25ml solvothermal reaction kettle, heat it to 180°C at a heating rate of 2°C / min, react for 6 hours, cool to room temperature naturally, suction filter, wash, dry and grind , to obtain black powder;

[0024] (3) Heat the black powder obtained in step (2) to 300°C at a heating rate of 2°C / min, react for 3 hours, cool to room temperature naturally, dry and grind to obtain Na 0.44 MnO 2 powder;

[0025] (4) 0.1g Na obtained in step (3) 0.44 MnO 2 Add the powder into 50ml 0.05mol / L sodium dodecylbenzenesulfonate aqueous solution, ultrasonically disperse for 30 minutes, add 0.0008g aniline monomer, stir for 20 minutes, add 0.002g (NH 4 ) 2 S 2 o 8 , reacted at 0°C for 6 hours, suction filtered, washed, dried and ground to obtain Na 0.44 MnO 2 Polyaniline composite...

Embodiment 2

[0027] (1) Add 0.23g (NH 4 ) 2 S 2 o 8 ,0.17g MnSO 4 ·H 2 O, 0.07g Na 2 SO 4 Add to 20g deionized water to make a uniform salt solution;

[0028] (2) Transfer the salt solution obtained in step (1) to a 25ml solvothermal reaction kettle, heat it to 180°C at a heating rate of 2°C / min, react for 6 hours, cool to room temperature naturally, suction filter, wash, dry and grind , to obtain black powder;

[0029] (3) Heat the black powder obtained in step (2) to 300°C at a heating rate of 2°C / min, react for 3 hours, cool to room temperature naturally, dry and grind to obtain Na 0.44 MnO 2 powder;

[0030] (4) 0.1g Na obtained in step (3) 0.44 MnO 2 Add the powder into 50ml 0.05mol / L sodium dodecylbenzenesulfonate aqueous solution, ultrasonically disperse for 30 minutes, add 0.0008g pyrrole monomer, stir for 20 minutes, add 0.003g (NH 4 ) 2 S 2 o 8 , reacted at 0°C for 6 hours, suction filtered, washed, dried and ground to obtain Na 0.44 MnO 2 polypyrrole composites...

Embodiment 3

[0032] (1) 1.8g (NH 4 ) 2 S 2 o 8 ,1.4g MnSO 4 ·H 2 O, 0.6g Na 2 SO 4 Add to 160g deionized water to make a uniform salt solution;

[0033] (2) Transfer the salt solution obtained in step (1) to a 200ml solvothermal reaction kettle, heat it to 180°C at a heating rate of 2°C / min, react for 8 hours, cool to room temperature naturally, suction filter, wash, dry and grind , to obtain black powder;

[0034] (3) Heat the black powder obtained in step (2) to 300°C at a heating rate of 2°C / min, react for 3 hours, cool to room temperature naturally, dry and grind to obtain Na 0.44 MnO 2 powder;

[0035] (4) 0.1g Na obtained in step (3) 0.44 MnO 2 Add the powder into 50ml of 0.05mol / L sodium dodecylbenzenesulfonate aqueous solution, ultrasonically disperse for 30 minutes, add 0.0008g of aniline monomer, stir for 20 minutes, add 0.0014g of ferric chloride, and react at 0°C for 6 hours. Suction filtration, washing, drying and grinding to obtain Na 0.44 MnO 2 Polyaniline com...

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Abstract

The invention discloses a preparation method of a sodium ion anode material. The anode material is a manganese oxide and conductive high polymer composite. The preparation method comprises the steps of preparing a manganese oxide crystal through hydrothermal reaction, and performing surface coating on the manganese oxide crystal with a conductive high polymer to form the sodium ion anode material. The shape of the prepared material is easy to control, the distribution is uniform, the coating is relatively uniform, a preparation process is simple, and the material is green and environment-friendly. According to the method, the manganese oxide is coated with the conductive high polymer, so that the manganese oxide is isolated from an electrolytic solution, and the first efficiency and cycling stability of the material are improved. The sodium ion anode material is excellent in rate capability, low in irreversible capacity and good in cycling performance.

Description

technical field [0001] The invention belongs to the field of electrochemistry, and also belongs to the field of energy technology, and in particular relates to a preparation method of a positive electrode material of a sodium ion battery. Background technique [0002] Currently, there is intense interest in developing inexpensive and safe energy conversion and storage devices. Due to the abundance of sodium in the earth's crust, its low price, and its electronic structure and chemical properties similar to lithium, sodium-ion secondary batteries are expected to be used in large-scale power grids and electric vehicles. One of the storage devices. [0003] The reported cathode materials for sodium-ion batteries such as olivine-structured NaFePO 4 、Na of NASICON structure 2 FePO 4 F and layered oxide Na x MO 2 (M=Co, Cr), etc., the theoretical specific capacity is low and the cycle performance is poor. Therefore, the development of cathode materials with good cycle perfo...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): H01M4/505
CPCY02E60/122H01M4/366H01M4/505H01M4/608H01M10/054Y02E60/10
Inventor 刘伟良周广盖邵光伟姚金水
Owner QILU UNIV OF TECH