Unlock instant, AI-driven research and patent intelligence for your innovation.

Method for preparing 3D iron--oxide/graphene composite electrode material of super capacitor

A graphene composite, supercapacitor technology, applied in the field of electrochemistry, can solve problems such as poor conductivity, achieve the effects of improved conductivity, high specific capacitance and rate characteristics, and improved cycle stability

Active Publication Date: 2017-02-15
嘉善县临沪新城实业有限公司
View PDF3 Cites 9 Cited by
  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Aiming at the problem of poor conductivity of iron oxide itself, by combining it with multiple graphite oxide gels to form an electron / ion conduction network of the composite material, the conductivity of the composite electrode material is significantly improved, thereby realizing a supercapacitor with high specific capacitance. Capacity and Rate Characteristics

Method used

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
View more

Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0026] Dissolve 600mg of polyvinylpyrrolidone in 800mL of methanol, add 590mg of ferric sulfate, ultrasonically disperse evenly, then add 2.63g of 4-nitroimidazole under stirring, stir in a water bath at 25°C for 1 hour, and let stand at room temperature for 24 hours to precipitate Iron-imidazole framework compound, washed with methanol and dried by centrifugation. The iron-imidazole framework compound in the Ar 2 / H 2 Heating at 350°C in the air for half an hour, and then calcining at 200°C in the air for half an hour to obtain iron oxide microspheres. Ultrasonic disperse iron oxide microspheres and graphite oxide (1:5) in 200mL of secondary water, add 3g of ascorbic acid, ultrasonically disperse for 2 hours, put it in a constant temperature water bath at 40°C, heat for 17 hours, put it in -4 overnight in the refrigerator at ℃, then freeze-dry to obtain a single iron oxide / graphite oxide airgel, puncture holes on the airgel, and introduce the above-mentioned iron oxide and ...

Embodiment 2

[0028] Dissolve 600mg of polyvinylpyrrolidone in 800mL of methanol, add 590mg of ferric chloride, ultrasonically disperse evenly, then add 2.63g of 2-nitroimidazole under stirring, stir in a water bath at 40°C for 2 hours, and let stand at room temperature for 24 hours , the iron-imidazole framework compound was precipitated, washed and dried by centrifugation with methanol. Iron-imidazole framework compound in Ar 2 / H 2 Heating at 350°C for 1 hour in the atmosphere, and then calcining at 500°C in the air for 5 hours to obtain iron oxide microspheres. Ultrasonic disperse iron oxide microspheres and graphite oxide (1:6) in 200mL of secondary water, add 3g of sodium borohydride, ultrasonically disperse for 2 hours, heat, put in a constant temperature water bath at 40°C, and heat for 17 hours. Put it in a -4°C refrigerator overnight, and then freeze-dry to obtain a single iron oxide / graphite oxide airgel. Puncture a hole on the airgel, and introduce the above-mentioned iron oxi...

Embodiment 3

[0030] Dissolve 600mg of polyvinylpyrrolidone in 800mL of methanol, add 590mg of ferric chloride, ultrasonically disperse evenly, then add 2.63g of 2-methylimidazole under stirring, stir in a water bath at 40°C for 1 hour, and let stand at room temperature for 24 hours , the iron-imidazole framework compound was precipitated, washed and dried by centrifugation with methanol. Iron-imidazole framework compound in Ar 2 / H 2Heat at 500°C in the air for half an hour, and then calcinate at 350°C in the air for 2 hours to obtain iron oxide microspheres. Ultrasonic disperse iron oxide microspheres and graphite oxide (1:5) in 200mL of secondary water, add 3g of ascorbic acid, ultrasonically disperse for 2 hours, put it in a constant temperature water bath at 40°C, heat for 17 hours, put it in -4 overnight in the refrigerator at ℃, then freeze-dry to obtain a single iron oxide / graphite oxide airgel, puncture holes on the airgel, and introduce the above-mentioned iron oxide and graphit...

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
Login to View More

PUM

No PUM Login to View More

Abstract

The invention, which belongs to the electrochemical field, relates to a method for preparing a 3D iron--oxide / graphene composite electrode material of a super capacitor. An iron source compound reacts with an imidazole compound to form an iron-imidazole frame compound; calcination is carried out in air to obtain an iron-oxide microsphere; the iron-oxide microsphere and graphite oxide are dispersed in water in an ultrasonic mode; a multi-iron-oxide / graphite-oxide aerogel is prepared by using a multi-gel method; high-temperature calcination is carried out in an atmosphere of inert to obtain a 3D iron--oxide / graphene composite electrode material; the 3D iron--oxide / graphene composite electrode material is mixed with acetylene black and teflon, the materials are stirred uniformly, and the mixed materials are coated on the surface of nickel foam to prepare a super capacitor electrode; and then the capacitance performance is tested at an electrochemical workstation. The composite electrode has high electron / ion conductivity; and the specific capacitance, the rate capability, and the cycling stability of the super capacitor are improved substantially.

Description

technical field [0001] The invention belongs to the field of electrochemistry, in particular to a method for preparing a supercapacitor 3D iron oxide / graphene composite electrode material Background technique [0002] As people pay more and more attention to energy and environmental issues, electric vehicles have increasingly become the center of research and development in the automotive industry. As a key component of electric vehicles, the power supply system must meet the requirements of high capacity and high power. At present, the energy density of the power battery has been improved, but its low power density limits the full performance of the power battery. The high specific power of the supercapacitor is a good supplement to the power battery. It can form a hybrid power system with a secondary battery with high energy density to effectively make up for the lack of specific power of the power battery. At the same time, the supercapacitor has the characteristics of ...

Claims

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
Login to View More

Application Information

Patent Timeline
no application Login to View More
Patent Type & Authority Applications(China)
IPC IPC(8): H01G11/86H01G11/26H01G11/30H01G11/46H01G11/32
CPCY02E60/13H01G11/86H01G11/26H01G11/30H01G11/32H01G11/46
Inventor 李在均王会影张芷菁
Owner 嘉善县临沪新城实业有限公司