Organic photoelectric device containing fused heterocyclic compound and application thereof
A technology for optoelectronic devices and compounds, which is applied in the fields of electric solid-state devices, photovoltaic power generation, electrical components, etc., and can solve the problems of complex supporting equipment, complex structure of OLED devices, and great influence on device yield.
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[0131] Preparation of intermediate materials
[0132]
[0133] O-A-S5 (4g) and 4-bromo-2-chlorodibenzofuran (3g) were completely dissolved in 120ml tetrahydrofuran in a 250ml round bottom flask under a nitrogen atmosphere, then 80ml of 2M aqueous sodium carbonate was added, and then Tetrakis-(triphenylphosphine)palladium (0.2 g), and the mixture was heated and stirred for 8 hours. After cooling to room temperature, the aqueous layer was removed. Add 100 ml of dichloromethane, and wash twice with 30 ml of saturated brine. The dichloromethane layer was dried over anhydrous magnesium sulfate, and concentrated in vacuo. Then, petroleum ether:dichloro (20:1~1:1) was used as eluent to purify and separate on a silica gel column to obtain compound OO-A-S6 (yield 79%). MS(ESI):534.1(M+H)
[0134] Similar to the synthetic steps of OO-A-S6, the following intermediate materials can be obtained:
[0135]
[0136] OS-A-S6: MS (ESI): 550.1 (M+H)
[0137]
[0138] OO-C-S6: MS (...
Embodiment 1
[0145] Embodiment 1: the preparation of compound OO-A-36
[0146]
[0147] After S3 (5 g) and biphenylaniline (3 g) were completely dissolved in xylene (80 ml) in a 100 ml round bottom flask under a nitrogen atmosphere, sodium tert-butoxide (4 g), bis(tri-tert Butylphosphine)palladium (0.1g), the mixture was heated to reflux for 5-10 hours. After cooling down to room temperature, remove the salt by filtration, concentrate the solvent in vacuo, and use petroleum ether: dichloromethane (20:1 ~ 2:1) as eluent to purify and separate on a silica gel column to obtain OO-A-36 ( Yield 74%). HRMS(ESI):743.2684(M+H)
Embodiment 2
[0148] Embodiment 2: the preparation of compound OO-A-49
[0149]
[0150] The preparation steps of compound OO-A-49 are similar to Example 1. Yield 78%, HRMS (ESI): 757.2477 (M+H).
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