A kind of photosensitive resin and its preparation method and application
A technology of photosensitive resin and structural unit, applied in the field of photosensitive resin and its preparation, can solve the problems of large difference, non-uniform residual film rate, low residual film stability and surface uniformity, etc., and achieves heat resistance and leveling. The effect of improving the heat resistance and leveling performance, improving the stability and uniformity of the residual film rate
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Synthetic example 1
[0076] This synthesis example provides a kind of photosensitive resin EMTB01 and preparation method thereof, specifically as follows:
[0077] (1) In a three-neck flask equipped with a stirrer, dropping funnel and thermometer, add 500mL of solvent propylene glycol methyl ether acetate, heat up to 90°C, and dissolve 100g of methyl methacrylate (R 1 For methyl) (Shanghai Aladdin Biochemical Technology Co., Ltd.), methacrylic acid 82g (R 2 is methyl) (Shanghai McLean Biochemical Technology Co., Ltd.), p-styrene polysiloxane 124g (m=10~100, R 3 is methyl, R 4 benzene ring) (BYK-022, Shanghai Yuyu New Material Co., Ltd.), 2-methyl-2-adamantyl methacrylate 92g (R 5 For methyl, Bailingwei Technology Co., Ltd.) and initiator azobisisobutyronitrile 5g (Bailingwei Technology Co., Ltd.) were added dropwise into the three-necked bottle, and the dropwise addition was completed in 2 hours, and the reaction was carried out for 10 hours;
[0078] (2) The temperature was raised to 110° C. t...
Synthetic example 2
[0081] The difference with Synthesis Example 1 is that methyl methacrylate is replaced by ethyl methacrylate (R 1 is ethyl), and methacrylic acid is replaced by ethacrylic acid (R 2 is ethyl), and the para-styrene polysiloxane is replaced by vinyl polysiloxane (R 3 for hydrogen, R 4 is a single bond), replace 2-methyl-2-adamantyl methacrylate with 2-ethyl-2-adamantyl ethyl acrylate (R 5 and R 6 Ethyl), the preparation obtains EMTB02, yield 90.6%;
[0082]Structural characterization: The resin EMTB02 was dissolved in tetrahydrofuran and characterized by Waters-Breeze GPC gel permeation chromatography. The weight average molecular weight Mw=17500 and PDI=1.116 were measured.
Synthetic example 3
[0084] The difference with Synthesis Example 1 is that methyl methacrylate is replaced by phenethyl methacrylate (R 1 is phenylethyl), and methacrylic acid is replaced by phenylethyl acrylate (R 2 is phenylethyl), and the p-position styrene polysiloxane is replaced by terminal vinyl styrene polysiloxane (R 3 is phenethyl, R 4 Ethylene), replace 2-methyl-2-adamantyl methacrylate with 2-phenethyl-2-adamantyl phenethyl acrylate (R 5 and R 6 Be phenethyl), prepare EMTB03, yield 90.23%;
[0085] Structural characterization: The resin EMTB03 was dissolved in tetrahydrofuran and characterized by Waters-Breeze GPC gel permeation chromatography. The weight average molecular weight Mw=16500 and PDI=1.212 were measured.
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