Unlock instant, AI-driven research and patent intelligence for your innovation.

Preparation method of xylose residue cellulose nanocrystals and composite hydrogel thereof

A composite hydrogel and cellulose technology, applied in the fields of chemical engineering and polymer materials, can solve the problems of low gel strength and poor toughness, and achieve good biocompatibility, excellent tensile strength and elongation, excellent The effect of anti-protein non-specific adsorption properties

Active Publication Date: 2020-07-24
中科如米(北京)生态农业科技发展有限公司 +1
View PDF4 Cites 7 Cited by
  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, artificially synthesized hydrogels usually have disadvantages such as low gel strength and poor toughness, which are difficult to meet the requirements of practical applications.

Method used

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
View more

Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0024] The xylose residue raw material is dried in a vacuum oven at room temperature and pulverized with a pulverizer, and the xylose residue powder passing through a 40-mesh sieve is collected for future use.

[0025] 0.2g of FeCl 3 Add 25ml of formic acid to 100ml of sulfuric acid solution with a concentration of 60wt%, stir at 70°C for 20min, then add 10g of xylose residue powder, stir well and continue to react at 70°C for 6h, after the reaction is completed, add 900ml of distilled water to carry out Dilute, then centrifuge the mixture at a speed of 10000r / min for 15min, pour out the supernatant to retain the solid content, add 100ml of water to it for dispersion, and centrifuge at a speed of 10000r / min for 15min to wash the precipitate , centrifugation was repeated three times to obtain lignin-containing cellulose nanocrystals. Then add the solid material to a sodium hydroxide solution with a concentration of 2wt%, ultrasonically disperse it for 15 minutes, and then stir...

Embodiment 2

[0028] The xylose residue raw material is dried in a vacuum oven at room temperature and pulverized with a pulverizer, and the xylose residue powder passing through a 40-mesh sieve is collected for future use.

[0029] 0.2g of FeCl 3 Add 25ml of formic acid to 100ml of sulfuric acid solution with a concentration of 60wt%, stir at 70°C for 20min, then add 10g of xylose residue powder, stir well and continue to react at 70°C for 6h, after the reaction is completed, add 900ml of distilled water to carry out Dilute, then centrifuge the mixture at a speed of 10000r / min for 15min, pour out the supernatant to retain the solid content, add 100ml of water to it for dispersion, and centrifuge at a speed of 10000r / min for 15min to wash the precipitate , centrifugation was repeated three times to obtain lignin-containing cellulose nanocrystals. Then add the solid material to a sodium hydroxide solution with a concentration of 2wt%, ultrasonically disperse it for 15 minutes, and then stir...

Embodiment 3

[0032] The xylose residue raw material is dried in a vacuum oven at room temperature and pulverized with a pulverizer, and the xylose residue powder passing through a 40-mesh sieve is collected for future use.

[0033] 0.2g of AlCl 3 Add 25ml of oxalic acid to 100ml of sulfuric acid solution with a concentration of 65wt%, stir at 70°C for 20min, then add 10g of xylose residue powder, stir well, continue to react at 70°C for 6h, and add 900ml of Dilute with distilled water, then centrifuge the mixture at a speed of 10000r / min for 15min, pour out the supernatant to retain the solid content, add 100ml of water to it for dispersion, and centrifuge at a speed of 10000r / min for 15min to wash The precipitate was centrifuged three times to obtain lignin-containing cellulose nanocrystals. Then add the solid material to a sodium hydroxide solution with a concentration of 2wt%, ultrasonically disperse it for 15 minutes, and then stir it at 70°C for 6 hours. Ultrasonic dispersion was ca...

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
Login to View More

PUM

PropertyMeasurementUnit
lengthaaaaaaaaaa
diameteraaaaaaaaaa
tensile strengthaaaaaaaaaa
Login to View More

Abstract

The invention discloses a preparation method of xylose residue cellulose nanocrystals and composite hydrogel thereof. The method comprises the following steps: drying and refining a xylose residue rawmaterial; carrying out mixed acid treatment and separation on the generated xylose residue powder to obtain cellulose nanocrystals containing lignin; carrying out alkali treatment to separate the cellulose nanocrystals from lignin; and adding the xylose residue cellulose nanocrystals into a solution containing a hydrophilic polymer monomer and an initiator, and carrying out polymerization crosslinking reaction under ultraviolet irradiation to obtain the xylose residue cellulose nanocrystals / polymer composite hydrogel. According to the invention, the xylose residue rich in crystalline cellulose is used as a biomass raw material for the first time, cellulose nanocrystals are successfully extracted through mixed acid treatment and alkali treatment methods, and the further prepared cellulosenanocrystal / polymer composite hydrogel has excellent tensile strength and protein pollution resistance and has a good application prospect in the fields of biological medicines, cosmetics, wearable equipment and the like.

Description

technical field [0001] The invention relates to a preparation method of xylose slag cellulose nanocrystal and a composite hydrogel thereof, belonging to the fields of chemical engineering and polymer materials. Background technique [0002] With the depletion of fossil energy such as coal and petroleum and the continuous deterioration of the ecological environment, the development and application of environmentally friendly renewable energy resources have increasingly attracted widespread attention in various fields. Lignocellulose is a valuable biomass resource with the largest reserves in nature and is cheap and easy to obtain. It is mainly composed of cellulose, hemicellulose and lignin. Among them, cellulose is a macromolecular polymer composed of glucose, which contains an amorphous region and a crystalline region inside. The non-crystalline region of cellulose can be hydrolyzed by strong acid hydrolysis, enzymatic hydrolysis and other methods to further obtain high cry...

Claims

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
Login to View More

Application Information

Patent Timeline
no application Login to View More
Patent Type & Authority Applications(China)
IPC IPC(8): C08B15/02C08F251/02C08F220/60C08F220/38C08F220/58C08F220/20C08F2/50B01J20/26B01J20/28B01J20/30
CPCB01J20/24B01J20/262B01J20/28004B01J20/28047C08B15/02C08F2/50C08F251/02C08F220/58C08F220/20
Inventor 苏荣欣丁国杰叶慧君陈绍煌齐崴
Owner 中科如米(北京)生态农业科技发展有限公司