Self-monitoring acrylic ester and preparation method and application thereof
A technology of acrylate and tetraphenylethylene monoacrylate, which is applied in the field of water-based acrylic resin coatings and their preparation, can solve problems such as crack growth and coating damage, and achieves the effects of low preparation cost, guaranteed safety, and convenient identification.
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Embodiment 1
[0027] This embodiment provides a preparation method of self-monitoring acrylate, the preparation method is as follows:
[0028] Excess dihydroxylated tetraphenylethylene ( figure 2 ) reacted with acrylate at 160±1°C, catalyzed by an aqueous sulfuric acid solution with a mass fraction greater than or equal to 70%, for 18 to 36 hours, and then obtained tetraphenylethylene monoacrylate ( image 3 ).
[0029] Tetraphenylethylene monoacrylate ( image 3 ) respectively with 1,6-dibromohexane (1,8-dibromooctane, 1,10 dibromodecane, 1,12-dibromododecane) in K 2 CO 3 React under catalysis for 10~15h, then column chromatography separates and obtains self-monitoring acrylate ( figure 1 ).
Embodiment 2
[0031] In this example, methyl methacrylate, butyl acrylate, crosslinking agent ethyl diacrylate, emulsifier sodium dodecyl sulfonate, and initiator potassium persulfate were all purchased from Beijing Yinuokai Reagent Co., Ltd.
[0032] The present embodiment comprises the preparation method of self-monitoring type waterborne acrylic resin coating, comprises the following steps:
[0033] (1) Pre-emulsification.
[0034] Use an electronic balance to weigh 80 parts of methyl methacrylate (relative mass, the same below), 150 parts of butyl acrylate, mix and configure monomer mixture A; then weigh 1 part of emulsifier sodium dodecylsulfonate and dissolve in 80 Parts of deionized water, stirred mechanically for 30 minutes until the emulsifier is completely dissolved, the stirring speed is 220r / min; then add 20% monomer mixture A, and stir for 30min at 70±5°C, the stirring speed is 220r / min.
[0035] (2) Monomer prepolymerization.
[0036] 3.2 parts of ammonium persulfate are dis...
Embodiment 3
[0040] In this example, methyl methacrylate, butyl acrylate, crosslinking agent ethyl diacrylate, emulsifier sodium dodecyl sulfonate, and initiator potassium persulfate were all purchased from Beijing Yinuokai Reagent Co., Ltd.
[0041] The present embodiment comprises the preparation method of self-monitoring type waterborne acrylic resin coating, comprises the following steps:
[0042] (1) Pre-emulsification.
[0043] Use an electronic balance to weigh 120 parts of methyl methacrylate (relative mass, the same below), 300 parts of butyl acrylate, mix and configure monomer mixture A; then weigh 0.5 parts of emulsifier sodium lauryl sulfonate and dissolve in 80 parts to remove Ionized water, stirred mechanically for 30 minutes until the emulsifier is completely dissolved, the stirring rate is 300r / min; then add 30% monomer mixture A, and stir for 50min at 70±5°C, the stirring rate is 300r / min.
[0044] (2) Monomer prepolymerization.
[0045] Dissolve 4 parts of ammonium pers...
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