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Preparation method of composite adhesive for antioxidant pipes

A technology for compounding adhesives and plastic pipes, applied in the direction of adhesives, epoxy resin adhesives, adhesive types, etc., can solve the problem of layering, co-extrusion surface bonding strength of single-layer pipe and barrier layer coating is low, etc. problems, to achieve the effect of improving wettability and adhesion, high bond energy, and improving viscosity

Pending Publication Date: 2019-08-16
陈光辉
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] The technical problem to be solved by the present invention: the co-extruded surface of the single-layer pipe and the barrier layer coating has low bonding strength and is prone to delamination

Method used

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Examples

Experimental program
Comparison scheme
Effect test

example 1

[0033] In parts by weight, weigh 5 parts of anhydrous calcium chloride, 60 parts of N-picoline, 10 parts of p-phenylenediamine, and 30 parts of terephthaloyl chloride, and add anhydrous calcium chloride to In N-methylpyridinone, stir at 100r / min in a water bath at 25°C for 25min to obtain an N-methylpyridinone solution, and add p-phenylenediamine to the N-methylpyridinone solution to obtain Inject nitrogen gas at an airflow rate of 20mL / min to remove oxygen, stir at 400r / min at room temperature for 25min, then place in ice water at 0°C for 3min to obtain a mixed solution, add terephthaloyl chloride to the mixed solution, Stir at room temperature at 400r / min for 5 minutes to obtain a gel. Incubate the gel at 140°C for 4 hours, beat the pulp, wash with water at room temperature for 5 minutes, and then boil it in 80°C hot water for 20 minutes. Dry for 3 hours to obtain aramid pulp, and then weigh 5 parts of trishydroxymethylaminomethane, 10 parts of dopamine hydrochloride, 40 par...

example 2

[0035] In parts by weight, weigh 10 parts of anhydrous calcium chloride, 80 parts of N-picoline, 20 parts of p-phenylenediamine, and 40 parts of terephthaloyl chloride, and add anhydrous calcium chloride to In N-methylpyridinone, stir at 100r / min in a water bath at 30°C for 30min to obtain an N-methylpyridinone solution, and add p-phenylenediamine to the N-methylpyridinone solution to obtain Inject nitrogen gas at an airflow rate of 30mL / min to remove oxygen, stir at room temperature at 500r / min for 30min, then place in ice water at 0°C for 5min to obtain a mixed solution, add terephthaloyl chloride to the mixed solution, Stir at room temperature at 500r / min for 10 minutes to obtain a gel. Incubate the gel at 150°C for 5 hours, beat the pulp, wash with water at room temperature for 10 minutes, and then boil it in hot water at 85°C for 30 minutes. Dry for 5 hours to get aramid pulp, and weigh 10 parts of tris-tris, 20 parts of dopamine hydrochloride, 60 parts of aramid pulp, an...

example 3

[0037] In parts by weight, weigh 7 parts of anhydrous calcium chloride, 70 parts of N-picoline, 15 parts of p-phenylenediamine, and 35 parts of terephthaloyl chloride, and add anhydrous calcium chloride to In N-methylpyridinone, stir at 100r / min in a water bath at 27°C for 27min to obtain an N-methylpyridinone solution, and add p-phenylenediamine to the N-methylpyridinone solution to obtain Inject nitrogen gas at an airflow rate of 25mL / min to remove oxygen, stir at room temperature at 450r / min for 27min, then place in ice water at 0°C for 4min to obtain a mixed solution, and add terephthaloyl chloride to the mixed solution, Stir at 450r / min at room temperature for 7 minutes to obtain a gel, incubate the gel at 145°C for 5 hours, make a pulp, wash with water at room temperature for 7 minutes, then boil in hot water at 87°C for 20 minutes, and then heat the gel at 120°C Dry for 5 hours to get aramid pulp, and then weigh 5 parts of tris-tris, 20 parts of dopamine hydrochloride, ...

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PUM

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Abstract

The invention relates to a preparation method of a composite adhesive for antioxidant pipes, and belongs to the field of adhesives. The solid adhesive is prepared by adding aramid fiber pulp into an elastomer. The main component of aramid fiber pulp is poly(p-phenylene terephthamide), and the bonding force between a plastic pipe and an antioxidant film is enhanced. Dopamine hydrochloride is adopted to modify aramid fiber pulp. Dopamine can carry out oxidation polymerization reactions in an oxygen containing alkaline water solution; after the reactions, a polydopamine layer with a strong adhesive performance is formed on the surface of a solid material; moreover, the polydopamine layer is rich in groups such as -NH2, -OH, catechol group, and the like, the activity of the solid surface is improved; at the same time, covalent-non-covalent interactions of the functional groups are established on the surface of the solid material, and the bonding force between the plastic pipe and the antioxidant film is strengthened.

Description

technical field [0001] The invention relates to a preparation method of a composite adhesive for oxygen-barrier plastic pipes, belonging to the technical field of adhesives. Background technique [0002] In recent years, floor heating systems have been widely used in China. Generally, floor heating systems require the same life span as buildings. However, ordinary plastic pipes have an obvious disadvantage that they cannot completely block the penetration of oxygen, which will cause a large amount of biological slime in the pipes. It will cause corrosion of the steel water supply system and eventually lead to damage to the entire water supply system. Therefore, plastic oxygen barrier pipes have been widely used in the laying of floor heating pipes in recent years. [0003] As we all know, the aging of plastics and metals is the result of the joint action of light, heat, oxygen, and fatigue. As far as light is concerned, the service life of plastics will be extended by 10-2...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C09J129/04C09J163/00C09J177/10C09J139/06C09J101/28C09J181/04C09J11/04C09J11/06C09J11/08D06M13/368C08G69/32D06M101/36
CPCC08G69/32C08K2003/387C08L2203/18C08L2205/035C08L2205/16C09J11/04C09J11/06C09J11/08C09J129/04D06M13/368D06M2101/36C08L63/00C08L77/10C08L39/06C08L1/286C08L81/04C08K13/02C08K5/098C08K5/053C08K3/38C08K3/346C08K5/42
Inventor 陈光辉
Owner 陈光辉