A kind of multifunctional hemostatic sponge and its preparation method and application
A hemostatic sponge and multi-functional technology, applied in applications, medical formulas, bandages, etc., can solve the problems of increased pain and mortality of the injured, increased difficulty of wound treatment, increased difficulty of surgery, etc., to avoid secondary bleeding, Effect of improving hemostasis safety and rapid hemostasis performance
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[0043]As mentioned above, there is an urgent need to prepare polymer materials for hemostasis that are safe, effective, environmentally friendly, and have high antibacterial properties. Based on this, the present inventors have conducted a lot of research on hemostatic polymer materials. The present inventors noticed that graphene oxide (GO), as a two-dimensional nano-carbon material, has the properties of hydrophilicity, electronegativity and easy modification. And GO nanosheets can activate Src kinase and release calcium ions from cells to trigger platelet aggregation and promote blood coagulation. The Chinese patent application number 201410262747.4 discloses a preparation method of a cross-linked graphene sponge and its application in trauma hemostasis, which is prepared by reacting graphene oxide with an amino cross-linking agent. The cross-linked graphene sponge has ultra-fast water absorption performance, can quickly enrich blood components, and achieve the effect of h...
Embodiment 1
[0082] (1) Preparation of methacryloyl chitosan MAC
[0083] Weigh 1.2g chitosan raw material (Mw=20000, the degree of deacetylation of chitosan is between 85%-99.9%) and dissolve it in 20mL of acetic acid solution (1%), add each chitosan repeatedly Unit 0.1 molar equivalent of methacrylic anhydride, and the mixture was reacted at room temperature for 1 hour under continuous shaking. The methacryloyl chitosan (DM=23%) was obtained by dialysis and freeze-drying.
[0084] (2) Preparation of cross-linked chitosan sponge CMS and multifunctional GO@CMS composite hemostatic sponge
[0085] Take the MAC prepared in step (1) and redissolve to obtain a 20mg / mL MAC solution, and then add graphene oxide solution, polyethylene glycol diacrylate (Mw=400) and MAC solution in a mass ratio of 4.5:2:1, It is guaranteed that graphene oxide accounts for 60% of the total system mass percentage. Add 1.5 mg / mL initiator to the system and react at 80°C for 2 hours to obtain a cross-linked product...
Embodiment 2
[0088] (1) Preparation of methacryloyl chitosan MAC
[0089] Weigh 1.2g chitosan raw material (Mw=50000, the degree of deacetylation of chitosan is between 85%-99.9%) and dissolve in 20mL of acetic acid solution (5%), add each chitosan repeatedly Unit 1 molar equivalent of methacrylic anhydride, the mixture was reacted at room temperature for 5 hours under continuous shaking. The methacryloyl chitosan (DM=35%) was obtained by dialysis and freeze-drying.
[0090] (2) Preparation of cross-linked chitosan sponge CMS and multifunctional GO@CMS composite hemostatic sponge
[0091] Take the MAC prepared in step (1) and redissolve to obtain a 30mg / mL MAC solution, and then add graphene oxide solution, polyethylene glycol diacrylate (Mw=800) and MAC solution in a mass ratio of 7:2:1, It is guaranteed that graphene oxide accounts for 70% of the total system mass percentage. Add 2mg / mL initiator to the system and react at 70°C for 4 hours to obtain a cross-linked product. After wash...
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