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Method for preparing high water absorption and water retention composite materials containing layer silicate mineral

A layered silicate and composite material technology, which is applied in the field of preparation of super water-absorbing and water-retaining composite materials, can solve the problems of short service life, high raw material and preparation costs, and easy mildew, and achieve low cost and good product performance , the effect of fast water absorption

Inactive Publication Date: 2008-09-17
CHINA UNIV OF GEOSCIENCES (WUHAN)
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Compared with the aqueous solution polymerization method, this method has many advantages, such as easy control of the reaction, small granular products, convenient post-processing, low energy consumption, and better product performance. However, since all monomers used in this method are acrylic acid, Raw materials and preparation costs are still high
CN1415696 adopts the inverse suspension method, utilizes gelatinized konjac powder to graft water-soluble vinyl monomers, and prepares soil water-retaining agent. This method effectively reduces the cost of raw materials, but because konjac powder is prone to mildew under the action of bacteria , so the prepared product is easy to degrade, and its actual service life is not long

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0037] Add 230ml of cyclohexane and 1.8g of Span-60 into the reactor, raise the temperature to 75°C, blow nitrogen to drive off the oxygen, and start stirring to completely dissolve the Span-60 to form an oil phase.

[0038] Dissolve 13.4 g of sodium hydroxide in 40 g of deionized water, and let it cool for a period of time or quickly cool it in ice water. Another 30g of acrylic acid was weighed, and the sodium hydroxide solution was slowly added dropwise to the acrylic acid in an ice-water bath with stirring to neutralize (that is, the degree of neutralization was 80%), so that the weight concentration of the monomer in the water phase was 25%. , then add 0.1g of potassium persulfate and 3g of kaolinite powder (content ≥ 40%, particle size ≤ 45um) after mechanical crushing, ultrasonically disperse with ultrasonic waves, after mixing evenly, slowly add the mixed monomer aqueous solution dropwise In the above oil phase, polymerize at 75°C for 2 hours, wait until the temperature...

Embodiment 2

[0040] Add 300ml of toluene and 0.7g of Span-60 into the reactor, raise the temperature to 75°C, blow nitrogen to drive off the oxygen, and start stirring to completely dissolve Span-60 to form an oil phase.

[0041] In 100 grams of acrylic acid solution with a concentration of 50% and a neutralization degree of 60%, add 20 grams of acrylamide, 0.007 grams of N, N'-methylenebisacrylamide and 0.425 grams of ammonium persulfate under stirring, dissolve, and then add Add 96 grams of mechanically pulverized talc (content ≥ 90%, particle size ≤ 45um) and ultrasonically disperse for 20 minutes. Under the condition of constant stirring, the mixed monomer aqueous solution was slowly added dropwise into the container containing the above oil phase, and polymerized at 70°C for 5h. When the temperature drops to room temperature, add methanol for dehydration, wash with ethanol, filter, and vacuum-dry the polymerized product at 80°C for 3 hours, then mechanically pulverize or not mechanica...

Embodiment 3

[0043] Add 480ml of cyclohexane and 1.8g of Span-60 into the reactor, raise the temperature to 75°C, blow nitrogen to drive off the oxygen, and stir to completely dissolve the Span-60 to form an oil phase.

[0044] Add 40 grams of acrylamide to 200 grams of methacrylic acid solution with a concentration of 40% and a neutralization degree of 90%, dissolve it, and add 0.024 grams of N, N'-methylenebisacrylamide, 0.115 sodium persulfate and peroxide under stirring. Dissolve 0.110 g of ammonium sulfate, then add 10 g of mechanically pulverized illite (content ≥ 60%, particle size ≤ 45 um), and disperse in a colloid mill. While maintaining constant stirring, slowly drop the mixed monomer aqueous solution into the container containing the above oil phase, and polymerize at 75°C for 3h. When the temperature drops to room temperature, add methanol for dehydration, wash with ethanol, filter, and dry the resulting gel at 110°C for 2 hours, then mechanically pulverize or without mechanic...

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PUM

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Abstract

The invention relates to a method for preparation of high water-absorbing and water-retaining composite containing non-metallic minerals. The method for preparation of high water-absorbing and water-retaining composite containing layered silicate mineral is characterized in that it consists of the following steps: 1) finely processed treatment of layered silicate mineral; 2) decentralized processing: adding the treated layered silicate mineral into the water-soluble vinyl unsaturated monomer solution with 5-50 % of weight concentration containing water-soluble free radical polymerization initiator and cross linker for decentralized processing; 3) polymerization reaction: slowly dripping the said compound into hydrophobic organic dispersed mediator dissolving surfactant or / and polymer protecting colloid, then performing water-in-oil anti-phase suspension polymerization at 20-90 DEG C for 1-6 hours; 4) after-treatment: after the said polymerization, when the temperature reduces to the room temperature, adding organic solvent for dehydration or azeotropic distillation dehydration,washing with alcohol, filtering, vacuum drying the polymerizate at 40-110 DEG C to obtain the product. The invention has characteristics such as low preparation cost and good combination property of the product.

Description

technical field [0001] The invention relates to a preparation method of a highly water-absorbing and water-retaining composite material containing non-metallic minerals, in particular to a preparation method of a highly water-absorbing and water-retaining material containing layered silicate minerals. Background technique [0002] In recent years, superabsorbent and water-retaining composite materials have been widely used in many fields such as agriculture, forestry and gardening, physiological hygiene, petroleum, chemical industry, building materials and food because of their excellent water absorption and water retention properties. However, traditional superabsorbent resins synthesized from water-soluble ethylenically unsaturated monomers (such as acrylic acid, acrylamide and vinyl alcohol) either have high raw material costs, low water absorption, or poor salt resistance. poor, which limits their application. The combination of hydrophilic inorganic non-metallic minera...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C08L101/02C08K3/34C08K9/00C08F2/32C08F2/44
Inventor 范力仁潘亚平田慧卿沈上越
Owner CHINA UNIV OF GEOSCIENCES (WUHAN)