Anti-melamine monoclonal antibody and application thereof
A monoclonal antibody and melamine technology, which is applied to instruments, peptides, immunoglobulins, etc., can solve the problems of high cost and time-consuming detection, and achieve the effects of saving time, simple operation, and strong specificity
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Embodiment 1
[0034] Embodiment 1, the preparation of melamine structural analogue (SM)
[0035] The molecular formula of SM is as follows:
[0036]
[0037] 1. Preparation and characterization of compound 3
[0038] 1. Preparation of Compound 3
[0039]
[0040] 2,3-dihydropyran (compound 1) (0.56g, 6.63mmol), 6-bromo-1-hexanol (1g, 5.52mmol) and pyridine p-toluenesulfonate (0.28g, 1.1mmol ) was dissolved in 15 mL of dichloromethane (DCM), and the reaction solution was stirred at room temperature for 23 hours. with saturated NaHCO 3 solution and saturated brine to wash the reaction solution, anhydrous Na 2 SO 4 dry. The desiccant was removed by filtration, and the solvent was distilled off under reduced pressure to obtain a colorless oily liquid compound 3 (1.4 g, yield 96%).
[0041] 2. Characterization of Compound 3
[0042] 1 HNMR (CDCl 3 , 400MHz) δ4.57(m, 1H), 3.86(m, 1H), 3.74(m, 1H), 3.50(m, 1H), 3.36-3.43(m, 3H), 1.82-1.91(m, 3H) , 1.71 (m, 1H), 1.38-1.64 (m, 10H). ...
Embodiment 2
[0087] Embodiment 2, the preparation of antigen
[0088] For the schematic diagram of antigen: SM-BSA (SM-KLH) coupling reaction, see figure 1 .
[0089] 1. Preparation of SM-BSA (coating antigen)
[0090] Weigh 5mg of SM and 20mg of BSA, fully dissolve in 5ml of hydrochloric acid acidified deionized water (pH4.7), add 46mg of EDC to the mixed solution, and react overnight under stirring at 4°C; It is 0.01M PBS buffer solution (pH7.0); respectively take BSA and SM-BSA with the same concentration (2mg / mL) for mass spectrometry analysis to identify the coupling results.
[0091] For mass spectrometry results, see figure 2 . The molecular weight of BSA is 66.32KD. The average molecular weight of SM-BSA is 70.57KD, an increase of 4.25KD compared with BSA. The molecular weight of SM is 221D. The formation of SM-BSA is through the dehydration of the carboxyl group on the SM side chain and the free amino group on the lysine on the surface of BSA through EDC to form an amide bo...
Embodiment 3
[0094] Embodiment 3, the preparation of monoclonal antibody
[0095] 1. Immunization of mice
[0096] 1. Five BALB / c mice aged 6-8 weeks were taken, and each mouse was subcutaneously injected with 20 μg of SM-KLH emulsified in complete Freund's adjuvant (primary immunization).
[0097] 2. Subcutaneous injection of the same dose of SM-KLH emulsified in Freund's incomplete adjuvant every 15 days (boosting immunization).
[0098] 3. Orbital blood was collected 10 days after the fourth immunization, the titer of antiserum was detected by indirect ELISA, and the specificity of the antibody relative to melamine was detected by indirect competitive ELISA.
[0099] The antiserum titers of 5 mice were all 1:72000. 1 # ,2 # 、3 # The antiserum of the mouse can recognize melamine more specifically than the antiserum of the other 2 mice; when adding the same dose of melamine, 3 # B / B of mouse antiserum 0 The smaller the value, the more obvious the suppression phenomenon.
[0100] 4....
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