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Method for separating clenobuterol hydrochloride through molecularly imprinted polymer

A clenbuterol hydrochloride and molecular imprinting technology, applied in the field of chemical engineering, can solve the problems of template residue and cross infection, and achieve the effects of high specificity and selectivity, improved sensitivity and high capacity

Inactive Publication Date: 2013-03-27
SHANGHAI JIAOTONG UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

This method also has the problem of template residue, and it will cause cross-infection problems in the enzyme-linked immunosorbent assay

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0034] 1. Preparation of Molecularly Imprinted Polymers

[0035]In step 1, 0.5 mol of the template molecule clenbuterol, the functional monomer methacrylic acid (MAA), and the crosslinking agent ethylene glycol dimethacrylate (EGDMA) were mixed according to a molar ratio of 1:2:15, Dissolve it in 6.5mL porogen (chloroform: acetonitrile = 3:10), put it into an ampoule, add 0.021g initiator azobisisobutyronitrile (AIBN), ultrasonicate for 10min, then fill with nitrogen for 5min, vacuum Sealed, 60 ° C water bath for 24 hours, obtained clenbuterol molecularly imprinted polymer;

[0036] Step 2: Take out the massive polymer, grind it with a mortar, sieve it with a sample sieve with a pore size of 38 μm, suspend it with acetone and discard the superfine particles. After drying the polymer, methanol: acetic acid (9:1, v / v) and methanol: formic acid (9:1, v / v) Soxhlet extraction were performed 3 times each to remove most of the template molecules, 6 hours each time, and finally Pure...

Embodiment 2

[0043] 1. Preparation of Molecularly Imprinted Polymers

[0044] In step 1, 0.5 mol of the template molecule clenbuterol, the functional monomer methacrylic acid (MAA), and the crosslinking agent ethylene glycol dimethacrylate (EGDMA) were mixed according to a molar ratio of 1:3:15, Dissolve in 5mL of porogen (acetonitrile: chloroform = 10:3), put it into an ampoule, add 0.021g of initiator azobisisobutyronitrile (AIBN), sonicate for 15min, then fill with nitrogen for 5min, and vacuum seal , in a 60°C water bath for 24 hours to obtain the clenbuterol molecularly imprinted polymer;

[0045] Step 2: Take out the massive polymer, grind it with a mortar, sieve it with a sample sieve with a pore size of 45 μm, suspend it with acetone and discard the superfine particles. After drying the polymer, methanol: acetic acid (9:1, v / v) and methanol: formic acid (9:1, v / v) were extracted by Soxhlet four times to remove most of the template molecules, each time for 5 h, and finally Pure me...

Embodiment 3

[0052] 1. Preparation of Molecularly Imprinted Polymers

[0053] Step 1, mix 0.5 mol of clenbuterol template, functional monomer methacrylic acid (MAA), and crosslinking agent ethylene glycol dimethacrylate (EGDMA) according to the molar ratio of 1:6:15, and dissolve Put it into 8mL porogen (acetonitrile: chloroform = 10:3), put it into an ampoule, add 0.021g of initiator azobisisobutyronitrile (AIBN), ultrasonication for 10min, then fill with nitrogen gas for 5min, and vacuum seal. Water bath at 60°C for 24 hours to obtain clenbuterol molecularly imprinted polymer;

[0054] Step 2, take out the massive polymer, grind it with a mortar, sieve it with a sample sieve with a pore size of 54 μm, suspend it with acetone and discard the superfine particles. After drying the polymer, methanol: acetic acid (9:1, v / v) and methanol: formic acid (9:1, v / v) were extracted by Soxhlet 6 times each to remove most of the template molecules, 4 hours each time, and finally Pure methanol was ex...

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Abstract

The invention relates to a method for separating clenobuterol hydrochloride through a molecularly imprinted polymer in the technical field of chemical engineering, wherein a preparation method comprises the following steps: mixing clenbuterol, methacrylic acid and ethylene glycol dimethacrylate according to the mol ratio of 1:2 to 6:15, dissolving into a pore forming agent, placing into an ampere bottle, adding an initiator, charging nitrogen gas after ultrasonic processing, carrying out vacuum sealing, and carrying out thermal-initiated polymerization to form a blocky polymer; taking out the blocky polymer, grinding and screening; and drying the polymer, and then removing a template through Soxhlet extraction, high-temperature processing and solvent elution. A separation method comprises the following steps: homogenizing the molecularly imprinted polymer, filling into a polypropylene solid phase extraction small column, respectively adding a polyethylene sieve plate at the upper end and the lower end of a filling, and compacting the filling; activating the solid phase extraction small column, leaching the solid phase extraction small column, eluting, and collecting the clenobuterol hydrochloride. The molecularly imprinted polymer prepared by the method has high selectivity and high specificity, can resist bad environments and can be coupled with ELISA.

Description

[0001] The present invention is patented by patent application number: 200810207771.2, patent application name: preparation of molecularly imprinted polymer and its method of separating clenbuterol hydrochloride, applicant: Shanghai Jiaotong University, application date: December 25, 2008 Divisional application. technical field [0002] The invention relates to a method in the technical field of chemical engineering, in particular to a method for separating clenbuterol hydrochloride by using a molecularly imprinted polymer. Background technique [0003] Clenbuterol hydrochloride (CLB for short) is a synthetic beta 2 -Adrenergic receptor agonists, also known as "Clenbuterol", "Cathantine", etc., are generally used in clinical practice as their hydrochloride. because of its β 2 - High receptor selectivity, strong effect, less side effects, early used in the prevention and treatment of human and animal bronchial asthma and convulsions, is an ideal anti-asthma drug, the most w...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C07C215/68C07C213/10B01D15/08
Inventor 张大兵郑素连武爱波
Owner SHANGHAI JIAOTONG UNIV