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Method for preparing magnesium iron aluminum composite material from sulfuric-acid slag

A technology of sulfuric acid slag and composite materials, which is applied in the field of refractory materials, can solve the problems of high cost and difficulty in the synthesis of iron-aluminum spinel, and achieve the effects of high pass rate, excellent thermal shock stability and good wear resistance

Inactive Publication Date: 2019-07-30
江苏诺明高温材料股份有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] Aiming at the problems existing in the prior art, the present invention discloses a magnesium-iron-aluminum composite material prepared by using sulfuric acid slag as a raw material. Utilizing the excellent kiln skin-hanging performance and structural flexibility of the magnesium-iron-aluminum composite material, it is applied to cement kiln firing Compared with the traditional periclase-aluminum spinel brick, it avoids the difficulty and high cost of the synthesis of alumina spinel. At the same time, the product of the present invention has different oxidation-reduction atmospheres in the firing process. Strong adaptability, high pass rate of products, can turn sulfuric acid waste residue into treasure, and its promotion has good social and economic benefits

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0027] (1) Grind the sulfuric acid slag with water to a certain particle size. After the slurry is evenly stirred, the material A is obtained through magnetic separation, and the material A is washed with water to obtain the material B. Grind material B and magnesite into fine powder with a particle size of 325 mesh, where w(B):w(magnesite)=(7~15)%:(86~94)%, plus 1% dextrin Dry powder, after mixing, grind for 6h-18h, add 3% binder, press into adobe, after drying, heat it under oxidizing atmosphere at 1450°C-1730°C for a certain period of time to obtain material C;

[0028] (2) In terms of mass percentage, 70% of material C, 20% of magnesia, 7% of fused magnesia-alumina spinel, and 3% of tabular corundum are mixed in proportion, and 3% of pulp solution is added as a binder. During production, first weigh various raw materials according to the proportion, mix them evenly, and get the mud material through mixing, and then press it into shape with a friction press. High temperatu...

Embodiment 2

[0032] The production technology of the present embodiment is identical with embodiment 1, and difference is:

[0033] In terms of mass percentage, 60% of material C, 25% of magnesia, 12% of fused magnesia-aluminum spinel, 3% of tabular corundum, and 3% of pulp solution are used as binders.

[0034] The material C has four particle sizes of 5-3mm, 3-1mm, 1-0mm and ≤0.088mm, the magnesia has two particle sizes of 1-0mm and ≤0.088mm, and the fused magnesia-aluminum spinel is 3-1mm, the particle size of the tabular alumina is 3-1mm.

[0035] The performance indicators of the obtained product are: apparent porosity 15.8%, bulk density 3.01g / cm3, normal temperature compressive strength 73MPa, load softening temperature greater than 1680°C, thermal shock stability (1100°C, water cooling) 15 times, and its corrosion resistance , oxidation-reduction resistance, creep resistance and kiln-hanging skin performance are all good.

Embodiment 3

[0037] Production technology is identical with embodiment 1, and difference is:

[0038] In terms of mass percentage, 50% of material C, 32% of magnesia, 13% of fused magnesia-aluminum spinel, 5% of tabular corundum, and 3% of pulp solution are used as a binder.

[0039] The material C has four particle sizes of 5-3mm, 3-1mm, 1-0mm and ≤0.088mm, the magnesia has two particle sizes of 3-1mm, 1-0mm and ≤0.088mm, and the fused magnesia The spinel is 3-1mm, and the particle size of the tabular alumina is 3-1mm.

[0040] The performance indicators of the obtained product are: apparent porosity 16.3%, bulk density 3.0g / cm3, normal temperature compressive strength 70MPa, load softening temperature greater than 1680°C, thermal shock stability (1100°C, water cooling) 14 times, and its corrosion resistance , oxidation-reduction resistance, creep resistance and kiln-hanging skin performance are all good.

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Abstract

The invention relates to a method for preparing a magnesium iron aluminum composite material from sulfuric-acid slag, and belongs to the field of fire-resistant materials. The method comprises the specific steps that 1, the sulfuric-acid slag is ground by adding water to form slurry, the slurry is uniformly stirred, after magnetic separation, a material A is obtained, and the material A is washedwith water and deslimed to obtain a material B; 2, the material B and magnesite are ground into fine powder respectively, the fine powder is mixed and ground together, a binding agent is added, greenbricks are obtained through pressing, and after drying, heat preservation is conducted in the high-temperature oxidizing atmosphere to obtain a material C; 3, the material C is broken and then mixed with magnesia, magnesium aluminate spinel and corundum, a binding agent is added, pressing formation is conducted, drying is conducted in a dry kiln, and heat preservation is conducted in a high-temperature tunnel kiln. The magnesium iron aluminum composite material has the excellent performance of being high in strength, high in thermal shock resistance, high in refractoriness under load, high inhigh-temperature creep property, high erosion resistance and anti-strip performance, high in cement adherence, high in anti-reduction and anti-oxidization capacity and the like, the sulfuric-acid slagwastes can be turned into valuable things, and recycling of the sulfuric-acid slag is achieved.

Description

technical field [0001] The invention relates to a preparation method of a magnesium-iron-aluminum composite material for cement kilns, belonging to the field of refractory materials. Background technique [0002] Sulfuric acid slag is the waste residue produced during the production of sulfuric acid by sulfuric acid production plants and phosphate fertilizer plants. According to statistics, every 1 ton of sulfuric acid is produced with about 0.8 tons of slag and a small amount of soot. Since the raw material for the production of industrial sulfuric acid is pyrite, the sulfuric acid slag contains a large amount of iron and other precious non-ferrous metals. According to the differences in the grade and coexisting components of pyrite in various places, the content of iron in cinder usually accounts for about 33-57% of the total weight of cinder, and silicon dioxide accounts for 10-24%. In addition, it is accompanied by Cu, Zn, Pb and Small amounts of precious metals, which...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C04B35/66C04B33/132
CPCC04B33/132C04B35/66Y02P40/60
Inventor 钱志明钱晶张军杰黄京衡
Owner 江苏诺明高温材料股份有限公司