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Silicon carbide whisker reinforced porous periclase-spinel-carbon filter and preparation method thereof

A silicon carbide whisker and periclase technology, applied in ceramic products, manufacturing tools, casting equipment, etc., can solve problems such as poor thermal shock stability, short service life, and poor effect of removing inclusions, so as to increase strength and improve Strength and thermal shock stability, effect of improving thermal shock stability

Active Publication Date: 2021-05-14
WUHAN UNIV OF SCI & TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] In summary, there are still some technical defects in the existing porous ceramic filter: the strength of the filter skeleton is low, the thermal shock stability is poor, and the service life is short; the surface of the filter skeleton is relatively dense, and the effect of removing inclusions is poor, especially The removal effect on small size inclusions is weak

Method used

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Examples

Experimental program
Comparison scheme
Effect test

preparation example Construction

[0062] Step 3, preparation of silicon carbide preform

[0063] According to the mass ratio of cyclohexane: allylhydrogenpolycarbosilane (2-12): 1, the cyclohexane and the allylhydrogenpolycarbosilane are placed in a stirrer and stirred for 5-10min, Then add a platinum complex solution accounting for the mass of the cyclohexane and the allylhydropolycarbosilane and 0.08-0.14 wt%, stir for 5-10 minutes, and turn off the mixer to obtain a mixed solution.

[0064] Then impregnate the polyurethane foam template in the mixed solution, take it out and squeeze it manually, repeat the dipping-manual extrusion process for 2 to 5 times; after taking it out, place it at room temperature for 24 to 36 hours, and place it at 1100 to 1300 ° C under a nitrogen atmosphere Keep it warm for 1-2 hours, and cool to room temperature to obtain a silicon carbide preform.

[0065] Step 4. Preparation of silicon carbide whisker reinforced porous periclase-spinel-carbon filter

[0066] Using 89-97wt% o...

Embodiment 1

[0089] A silicon carbide whisker reinforced porous periclase-spinel-carbon filter and a preparation method thereof. The steps of the preparation method described in this specific embodiment are:

[0090] Step 1, preparation of porous periclase-spinel ceramic fine powder

[0091] Step 1.1. Heat the aluminum hydroxide fine powder to 370° C. at a rate of 2.5° C. / min, keep it warm for 1 hour, and cool to obtain alumina fine powder with high porosity.

[0092] Step 1.2: Stir 40wt% of the high-porosity alumina fine powder and 75wt% light-burned magnesite fine powder in a mixer for 3 hours to obtain a mixture I.

[0093] Step 1.3. According to the mass ratio of the mixture I: aluminum sol is 100:6, mix the mixture I and the aluminum sol for 13 minutes to obtain the mixture II. The mixture II was machine-pressed at 135 MPa, dried at 110°C for 36 hours, heated to 1750°C at a rate of 5°C / min, and kept for 6 hours to obtain porous periclase-spinel with micro-nano pores Ceramic materia...

Embodiment 2

[0119] A silicon carbide whisker reinforced porous periclase-spinel-carbon filter and a preparation method thereof. The steps of the preparation method described in this specific embodiment are:

[0120] Step 1, preparation of porous periclase-spinel ceramic fine powder

[0121] Step 1.1. Heat up the aluminum hydroxide fine powder to 390° C. at a rate of 2° C. / min, keep it warm for 3 hours, and cool to obtain alumina fine powder with high porosity.

[0122] Step 1.2: Stir 10 wt% of the high-porosity alumina fine powder and 90 wt% light-burned magnesite fine powder in a mixer for 1 hour to obtain a mixture I.

[0123] Step 1.3. According to the mass ratio of the mixture I: aluminum sol is 100:4, mix the mixture I and the aluminum sol for 18 minutes to obtain the mixture II. The mixture II was machine-pressed at 100 MPa, dried at 110°C for 18 hours, heated to 1720°C at a rate of 4°C / min, and kept for 2 hours to obtain porous periclase-spinel with micro-nano pores Ceramic mate...

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Abstract

The invention relates to a silicon carbide whisker reinforced porous periclase-spinel-carbon filter and a preparation method thereof. According to the technical scheme, the preparation method comprises the following steps: mixing porous periclase-spinel ceramic fine powder with a micro-nano aperture with a modified solution in a vacuum device, and drying; mixing the dried modified porous periclase-spinel ceramic fine powder with monatomic silicon powder, modified coal tar pitch powder, a water reducing agent, a rheological agent, aluminum sol, a defoaming agent and deionized water, and stirring to obtain slurry; immersing a silicon carbide preform into the slurry, standing, and carrying out centrifugal treatment to obtain a ceramic biscuit; and drying the ceramic biscuit, heating to 1350-1450 DEG C under a carbon burying condition, preserving heat, and cooling to obtain the silicon carbide whisker reinforced porous periclase-spinel-carbon filter. The silicon carbide whisker reinforced porous periclase-spinel-carbon filter prepared by the invention is high in strength, excellent in thermal shock resistance, long in service life and good in molten steel purification effect; and the filter is suitable for ultra-clean molten steel filtration.

Description

technical field [0001] The invention belongs to the technical field of porous ceramic filters. In particular, it relates to a silicon carbide whisker reinforced porous periclase-spinel-carbon filter and a preparation method thereof. Background technique [0002] Non-metallic inclusions in molten steel are the key factors affecting steel quality. Therefore, removing inclusions in molten steel and improving the cleanliness of molten steel are important technical means for producing high value-added steel products. Introducing a ceramic filter with a three-dimensional network skeleton structure and through-shaped pores at the final stage of molten steel pouring can effectively filter out inclusions in molten steel, and is an important method to purify molten steel and improve steel quality. [0003] At present, there have been many reports on the preparation of porous ceramic filters, such as "a magnesia-alumina spinel reinforced magnesium oxide-based foam ceramic filter and i...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C04B38/06C04B35/66B22D43/00B22C9/08
CPCC04B38/0615C04B35/66B22C9/086B22D43/004C04B2235/3206C04B2235/3222C04B2235/422C04B2235/3218C04B2235/442C04B2235/5276C04B2235/483C04B2235/428C04B2235/443C04B2235/77C04B2235/96C04B38/0067C04B38/0074Y02P10/20
Inventor 鄢文高仲钰陈哲王强刘昱李光强
Owner WUHAN UNIV OF SCI & TECH