A method for removing diclofenac in water by ferrite magnetic nanoparticles
A technology of magnetic nanoparticles and diclofenac, applied in separation methods, chemical instruments and methods, magnetic/electric field water/sewage treatment, etc., can solve the problems of secondary pollutants, increase energy consumption and cost, and achieve good removal effect, Large specific surface area and high activity, the effect of simple reaction conditions
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Embodiment 1
[0034] Nickel Ferrite (NiFe 2 o 4 ) magnetic nanoparticles to remove diclofenac in sewage
[0035]Add the diclofenac sewage water sample containing 10mg / L into the centrifuge tube, adjust the pH value of the water sample to 4±0.2 with sodium hydroxide or hydrochloric acid, and then add nickel ferrite magnetic nanoparticles at a dosage of 0.5g / L . Under the condition of room temperature, shake and react at a speed of 30 rpm for 2 hours, and after adsorption equilibrium, the nickel ferrite magnetic nanoparticles are separated by a magnet. The concentration of diclofenac in the treated water sample was analyzed by high performance liquid chromatography, and the removal rate reached 98.8%.
Embodiment 2
[0037] Manganese ferrite (MnFe 2 o 4 ) magnetic nanoparticles to remove diclofenac from surface water
[0038] With the method of embodiment 1, the difference is that the treated water sample is surface water, the adsorbent used is manganese ferrite magnetic nanoparticles, sodium hydroxide or hydrochloric acid is used to adjust the pH value of the water sample to 6 ± 0.2, and use high performance liquid chromatography The concentration of diclofenac in the treated water sample was analyzed by an instrument, and the removal rate was 93.9%.
Embodiment 3
[0040] Removal of diclofenac in drinking water by nickel ferrite magnetic nanoparticles
[0041] Using the method of Example 1, the difference is that the treated water sample is drinking water spiked water sample, the concentration of diclofenac is 1.5mg / L, the dosage of nickel ferrite magnetic nanoparticles is 0.1g / L, sodium hydroxide or The pH value of the water sample was adjusted by hydrochloric acid to 7±0.2, and the concentration of diclofenac in the treated water sample was analyzed by high performance liquid chromatography, and the removal rate was greater than 99.6%.
[0042] Through experiments and analysis tests of the present invention, when the nickel ferrite and the manganese ferrite remove diclofenac in the water sample, the reaction rate is fast, and the pH value of the water sample and the natural organic matter (humic acid concentration 0-20mg / L) are little affected, And can be reused. The specific experimental conditions are as follows:
[0043] (1) Adsor...
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