Polymer materials with electrostatic dissipative properties
a technology of polymer materials and dissipative agents, applied in the direction of circuit electrostatic discharge protection, synthetic resin layered products, transportation and packaging, etc., can solve the problems of serious accidents, unsatisfactory static electrical charge, plastic materials have a tendency to accumulate static electrical charge, etc., and achieve the effect of propagating charg
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example 1
Ferrocene-Containing Hydroxyl Terminated (FCOH) Prepolymer Synthesis
[0061] A scheme for the synthesis of 1,1′-di(chlorocarbonyl) ferrocene is shown in FIG. 7. To the solution of 4.0 g (0.013 mole) 1,1′-di(chlorocarbonyl) ferrocene in dry benzene (95 ml), 1.82 g (0.0154 mole) 1,6-hexanediol and pyridine (1.1 ml) was added. The mixture was stirred at 70-75° C. under an inert atmosphere (N2 gas) for 4 hours. The pyridinium chloride salt, being insoluble in benzene was precipitated from the reaction phase. The mixture was filtered and the solvent was evaporated under reduced pressure. The residue was extracted with CH2Cl2 and washed with water. The organic layer was dried (Na2SO4) and evaporated to give 4.3 g (88%) of ferrocene containing hydroxyl terminated prepolymer, FcOH. 1H NMR of this compound showed an average molecular weight of −3600. 1H NMR δ: 4.83 (s, 4H), 4.40 (s, 4H), 4.24 (t, 4H), 3.68 (t, 0.43H), 1.78 (m, 4H), 1.52 (m, 4H). IR (cm−1, neat): 1722.9 (C═O), 2940.4 (CH aliph...
example 2
FCOH-Containing Block Copolyurethanes
[0062] Block copolymers were prepared by using the “prepolymer method.” The diisocyanate-terminated prepolymer (BAYTEC ME-080, Bayer Corporation, Pa.) was heated at 100-110° C. for about 30 minutes (diphenylmethane-4,4′-diisocyanate (MDI) / polytetramethylene ether glycol (PTMEG) based BAYTEC ME-080 prepolymers, with NCO content of 8.64%). To this, FcOH dissolved in tetrahydrofuran (THF) and several drops of T-12 catalyst solution (dibutyltin dilaurate) were added. The mixture was mechanically stirred under nitrogen for 20 minutes, and then HDO was added and stirred for one minute. The films were cast from THF, on TEFLON sheets, and were cured under vacuum at 80° C. for 6 hours.
example 3
Ferrocene-Containing Amine Terminated (FcNH2) Prepolymer Synthesis
[0063] To the solution of 7.0 g (0.023 mole) 1,1′-di(chlorocarbonyl) ferrocene in CH2Cl2 (70 ml), 3.1 g (0.027 mole) 1,6-hexanediamine and 1.8 g (0.045 mole) NaOH dissolved in H2O (30 ml) was added at one portion and stirred vigorously for 10 minutes. The precipitate was filtered and washed with CH2Cl2 to give 9.0 g (93%) of FcNH2. Molecular weight by end group analysis was 1381. IR (cm−1, KBr pellet): 1551 (amide II band), 1637.3 (amide I band), 2868.0 and 2940 (CH aliphatic), 3091.8 (CH olefin), 3309.0 (NH). A scheme for the synthesis of ferrocene-containing amine terminated (FcNH2) prepolymer is shown in FIG. 9.
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