Heavy-oil hydrogenating catalyst and application thereof
A heavy oil hydrogenation and catalyst technology, applied in physical/chemical process catalysts, catalyst carriers, chemical instruments and methods, etc., can solve problems such as stable operation effects and achieve the effect of performance improvement
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[0012] Wherein, the preparation method of pseudo-boehmite P1 with 1.1≤n≤2.5 includes: contacting an aluminum-containing compound solution with an acid or alkali for precipitation reaction, or contacting an organic aluminum-containing compound with water for hydrolysis reaction to obtain a hydrated Alumina: aging the hydrated alumina obtained above, wherein any one of the contacting of the aluminum-containing compound solution with acid or alkali or the contacting of the organic aluminum-containing compound with water and the aging of the hydrated alumina It is carried out in the presence of a grain growth regulator, which is a substance capable of regulating the growth rate of crystal grains on different crystal planes.
[0013] Although the object of the present invention can be achieved as long as any one of the hydrolysis reaction or the precipitation reaction and the aging process is carried out in the presence of a grain growth regulator, preferably, the hydrolysis reactio...
Embodiment 1
[0049] (1) Boron-containing pseudoboehmite
[0050] In a 2-liter reaction tank, add 600 milliliters of concentration and be 96 grams of alumina / liter, aluminum sulfate solution containing 3.6 grams of ribitol and ammonia solution of 8% by weight to carry out precipitation reaction in parallel, and the reaction temperature is 40 ℃ , the reaction time is 10 minutes, the flow rate of the ammonia solution is controlled so that the pH of the reaction system is 7, after the precipitation reaction is finished, ammonia water is added in the slurry to make the pH of the slurry to be 8.5, and the slurry is aged at 55°C for 60 minutes and then filtered. The cake was beaten and washed twice with deionized water, and the filter cake was dried at 120°C for 24 hours to obtain hydrated alumina. Mix the obtained hydrated alumina with 60 mL of boric acid aqueous solution with a concentration of 19.2 g diboron trioxide / liter, and dry at 120°C for 12 hours to obtain boron-containing hydrated alum...
Embodiment 2
[0061] (1) Boron-containing pseudoboehmite
[0062] High-concentration NaAlO containing 210 grams of alumina / liter and a caustic coefficient of 1.62 2 solution with deionized water to prepare Al 2 o 3Concentration is 5 liters of solution of 40 grams / liter, then adds 16.3 grams of sodium gluconate to obtain NaAlO containing sodium gluconate 2 solution, and then transferred to a gelling reactor with a total volume of 8L, the ratio of height to diameter of the reactor is 8, and the lower part is equipped with CO 2 gas distributor. Control the temperature of the solution at 25±5°C, and feed CO with a concentration of 90% by volume from the bottom of the reactor 2 The gas carries out the gelation reaction, the gelation temperature is controlled at 20-40°C, and the CO 2 The gas flow rate is 15±2 liters / minute, and the pH value at the end of the reaction reaches 8.0-8.5 within 4-6 minutes, that is, the aeration is stopped, and the gelation reaction is ended. The obtained slurry...
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