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Solid polyacrylate resin containing anhydride functional group and preparation and use method thereof

A polyacrylate and acrylate technology, used in polyester coatings, epoxy coatings, coatings, etc., can solve the problem of affecting curing temperature and time window, affecting extinction, curing effect, low gloss and dead light, etc. problems, to achieve the effect of eliminating paint film defects, matting paint film defects, and improving appearance performance

Inactive Publication Date: 2021-07-16
ANSHAN RUNDE FINE CHEM
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0003] 1. Because it contains high polar functional groups such as carboxyl groups, the resin has high viscosity, especially the high acid value (AV>100) varieties, which brings many restrictions to its production and application; 2. Due to the low reactivity of carboxyl groups , and react with hydroxyl functional groups to generate small molecule water, which escapes when heated and cured, which affects the curing temperature and time window (requires high temperature baking and longer baking time) and the appearance of the paint film (prone to pinholes) , craters and other paint film defects); 3. Because the reactivity of carboxyl groups and their distribution characteristics in polyacrylate resin polymers affect their matting and curing effects, they cannot be used to produce powder coatings with extremely low gloss and dead light Variety

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0040] A kind of acrylate resin containing anhydride group functional group, the preparation method is as follows:

[0041] 1) Heat 100mL of toluene to 85°C under nitrogen protection;

[0042] 2) Mix 1.2g of initiator azobisisobutyronitrile and 1g of molecular weight regulator with 10g of tetrahydrophthalic anhydride, 10g of isobornyl acrylate, 10g of styrene, 40g of methyl methacrylate and 30g of methyl acrylate to obtain a mixed solution ;

[0043] 3) Keep the solvent temperature at 85°C, add the mixed solution obtained in step 2) to toluene dropwise for 5 hours; after the dropwise addition, continue to keep warm for 30 minutes;

[0044] 4) Add 0.3 g of azobisisobutyronitrile dissolved in 10 ml of toluene to the reaction solution, and continue to keep warm for 4 hours;

[0045] 5) After the reaction, the temperature was raised to 150°C, the solvent was evaporated, the temperature was lowered to 120°C, and the material was discharged under nitrogen protection. The material ...

Embodiment 2

[0049] A kind of acrylate resin containing anhydride group functional group, the preparation method is as follows:

[0050] 1) Heat 100ml of toluene and xylene (1:1v / v) mixed solution to 120°C under nitrogen protection;

[0051]2) Mix 1.1g of initiator benzoyl peroxide and 0.6g of molecular weight regulator with 10g of methyl nadic acid anhydride, 30g of isobornyl methacrylate, 25g of tertiary vinyl carbonate, 20g of n-butyl methacrylate and n-butyl acrylate 15 g of butyl esters were mixed to obtain a mixed solution;

[0052] 3) Keep the solvent temperature at 120°C, add the mixed solution obtained in step 2) into the solvent dropwise, and the dropwise addition time is 4 hours; after the addition, continue to keep warm for 45 minutes;

[0053] 4) Add 0.2 g of benzoyl peroxide solution dissolved in 10 ml of toluene to the reaction solution, and continue to keep warm for 2 hours;

[0054] 5) After the reaction, raise the temperature to 190°C, evaporate the solvent, cool down t...

Embodiment 3

[0058] A kind of acrylate resin containing anhydride group functional group, the preparation method is as follows:

[0059] 1) Heat 100ml butyl acetate to 110°C under nitrogen protection;

[0060] 2) Mix 1.7g of initiator azobisisobutyronitrile and 0.8g of molecular weight regulator with 10g of nadic anhydride, 10g of methyl nadic anhydride, 15g of isobornyl acrylate, 15g of isobornyl methacrylate, and 10g of styrene, Vinyl tertiary carbonate 5g, ethyl methacrylate 10g, n-butyl methacrylate 10g, ethyl acrylate 10g, and isooctyl acrylate 5g were mixed to obtain a mixed solution;

[0061] 3) Keep the solvent temperature at 103°C, add the mixed solution obtained in step 2) into the solvent dropwise for 6 hours; after the addition is complete, continue the heat preservation reaction for 40 minutes;

[0062] 4) Add 0.25 g of azobisisobutyronitrile dissolved in 10 ml of butyl acetate to the reaction solution, and continue to keep warm for 3 hours;

[0063] 5) After the reaction, t...

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Abstract

The invention aims to provide solid polyacrylate resin containing an anhydride functional group as well as a preparation method and a use method of the solid polyacrylate resin. The resin is prepared by taking an unsaturated anhydride functional monomer, a methacrylate monomer, an acrylate monomer, isobornyl acrylate and / or isobornyl methacrylate as well as styrene and / or a vinyl versatate monomer as raw materials through copolymerization by adopting a free radical solution polymerization method. According to the invention, the resin is matched with solid epoxy resin or a mixed epoxy resin system, a TGIC powder coating system and an HAA powder coating system for use, and realizes a series of functions, such as curing, extinction, paint film defect elimination and the like.

Description

technical field [0001] The invention belongs to the technical field of powder coating material synthesis, and in particular relates to a solid polyacrylate resin containing anhydride group functional groups and a preparation and use method thereof. Background technique [0002] Carboxyl type solid polyacrylate resin is an important functional application powder in powder coatings. It is used together with hydroxyl type polyester resin, epoxy and mixed epoxy resin, epoxy type acrylic resin, etc. to provide functions such as curing and matting, especially It is a solid acrylate resin with good decorative properties, aging resistance, high hardness and scratch resistance, making it an irreplaceable component in powder coatings. Its conventional synthesis method is the method of free radical solution polymerization. Acrylic acid, methacrylic acid carboxyl type functional monomers and hard monomers (methacrylates, (meth)acrylic acid-isopropyl esters, styrene propylene, etc.), sof...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C08F220/14C08F220/18C08F222/04C08F218/10C08F222/06C08F212/08C08F2/06C08F2/38C09D167/00C09D5/03C09D7/42C09D7/65C09D163/02C09D133/12C09D133/10C09D133/08C08G59/42
CPCC08F220/14C08F220/1811C08F220/1804C08F220/1802C08F222/04C08F2/06C08F2/38C09D133/064C09D163/00C09D167/00C09D5/033C08G59/4215C08K2003/2241C08K2003/3045C08L2205/03
Inventor 柳问林叶维德李文龙张琪雯汪海燕华正卫徐红玲
Owner ANSHAN RUNDE FINE CHEM