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Synthesis method of waterborne polyurethane primer

A technology of water-based polyurethane and synthesis method, used in polyurea/polyurethane coatings, coatings, primers, etc., can solve the problems of low bonding strength and poor stability, and achieve high solid content, good stability, and improved water resistance. Effect

Inactive Publication Date: 2020-03-06
SHANXI INST OF COAL CHEM CHINESE ACAD OF SCI
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] The purpose of the present invention is to overcome the shortcoming of prior art, provide a kind of synthetic method of water-based polyurethane primer, solve the technical problems such as poor stability, low bonding strength that existing water-based polyurethane primer exists

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0052] 1) 50g of dehydrated polycarbonate diol (molecular weight: 2000), 2.24g of dimethylolpropionic acid containing carboxylic acid groups, 22.64g of isophorone diisocyanate (IPDI) and 2.67g of 1,6-hexyl Add diisocyanate into the reactor, heat to 85°C during the stirring process and keep it warm for 1 hour, add 20g of acetone and 0.03g of catalyst dibutyltin dilaurate (T-12) and continue the reaction for 1h, then add 2.0g of 1,4 -Butanediol (BDO) and 20g of acetone, then react at 60°C for 2 hours, use di-n-butylamine back titration to analyze the NCO% content reaches the theoretical value, then cool down to 50°C, add 1.69g of triethylamine to neutralize For 20 minutes, the temperature was lowered to 40°C at the same time to obtain the intermediate;

[0053] 2) Add 9.8g of 50wt% sodium ethylenediamine sulfonate aqueous solution to the above-mentioned intermediate and stir rapidly for 10 minutes, then add deionized water and 5.4g of 3-ammonia Propyltriethoxysilane (KH550) and...

Embodiment 2

[0056] 1) 50g of dehydrated polycarbonate diol (molecular weight: 2000), 2.24g of dimethylolpropionic acid containing carboxylic acid groups, 22.64g of isophorone diisocyanate (IPDI) and 2.67g of 1,6-hexyl Add diisocyanate into the reactor, heat to 85°C during the stirring process and keep it warm for 1 hour, add 20g of acetone and 0.03g of catalyst dibutyltin dilaurate (T-12) and continue the reaction for 1h, then add 2.36g of diethylene glycol Alcohol (DEG) and 20g of acetone were reacted at 60°C for 2 hours, and the NCO% content was analyzed by di-n-butylamine back titration method to reach the theoretical value. After that, the temperature was lowered to 50°C, and 1.69g of triethylamine was added for neutralization for 20 minutes. At the same time, the temperature was lowered to 40° C. to obtain the intermediate;

[0057] 2) Add 9.8g of 50wt% sodium ethylenediamine sulfonate aqueous solution to the above-mentioned intermediate and stir rapidly for 10 minutes, then add deio...

Embodiment 3

[0060] 1) 50g of dehydrated polycarbonate diol (molecular weight is 2000), 2.24g of dimethylol propionic acid containing carboxylic acid groups, 26.7g of 4,4'-dicyclohexylmethane diisocyanate (H 12 MDI) and 2.67g of 1,6-hexamethylene diisocyanate were added to the reactor, heated to 85°C during the stirring process and kept for 1 hour of reaction, adding 20g of acetone and 0.03g of catalyst dibutyltin dilaurate (T-12) and continuing React for 1 hour, then add 2.63g of 1,6-hexanediol (HDO) and 20g of acetone, then react at 60°C for 2 hours, use di-n-butylamine back titration to analyze the NCO% content and reach the theoretical value, then cool down to 50°C , add 1.69g triethylamine to neutralize for 20 minutes, while cooling down to 40°C to obtain the intermediate;

[0061] 2) Add 9.8g of 50wt% sodium ethylenediamine sulfonate aqueous solution to the above-mentioned intermediate and stir rapidly for 10 minutes, then add deionized water and 3.54g of 3-ammonia Propyltriethoxysi...

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Abstract

The invention relates to a synthesis method of a waterborne polyurethane primer, and belongs to the technical field of synthesis methods of waterborne polyurethane primers. The technical problems of poor stability, low bonding strength and the like of existing waterborne polyurethane primers are mainly solved. The synthesis method of the waterborne polyurethane primer comprises the following steps: (1) adding a dehydrated polyol, an ion-radical-containing diol chain extender and a diisocyanate into a reactor, carrying out a reaction continuously after a solvent-1 and a catalyst are added, thenadding a small-molecule diol chain extender and a solvent-2, and adding a neutralizer for neutralization to obtain an intermediate; (2) adding an aqueous solution of a sulfonyl-group-containing diamine chain extender into the intermediate, then under fast stirring, adding deionized water for even dispersion, then adding a coupling agent and an aqueous solution of a small-molecule diamine chain extender for a chain extension reaction, and removing the solvents at vacuum to obtain waterborne polyurethane dispersion liquid; and (3) producing the waterborne polyurethane dispersion liquid and an assistant into the primer with proper viscosity and wettability.

Description

technical field [0001] The invention belongs to the technical field of synthesis methods of water-based polyurethane primers, in particular to a synthesis method of water-based polyurethane primers. Background technique [0002] Waterborne polyurethane (WPU) is increasingly widely used in coatings, adhesives, inks, etc. due to its environmental friendliness, low VOC emissions, and excellent comprehensive performance comparable to solvent-based polyurethanes. But there are also many disadvantages such as poor chemical resistance, thermal stability, mechanical properties and hydrolytic stability, which limit its application in various fields. Therefore, the research on improving WPU performance has always been a research hotspot. [0003] Organosiloxane resin has low surface tension, unique flexibility, low glass transition temperature, high temperature stability, good water resistance, chemical resistance and electrical insulation, but its cohesive energy density is low, att...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C08G18/66C08G18/44C08G18/34C08G18/32C08G18/28C08G18/12C09D175/06C09D5/00
CPCC08G18/12C08G18/289C08G18/3206C08G18/348C08G18/3855C08G18/44C08G18/6659C09D5/002C09D175/06
Inventor 赵雨花王军威亢茂青冯月兰殷宁李其峰张清运梁辰李晓云
Owner SHANXI INST OF COAL CHEM CHINESE ACAD OF SCI