Polymer matrix composite dielectric material and preparation method thereof
A composite material and polymer technology, which is applied in the field of composite dielectric film preparation, can solve the problems of polymer flexibility and processability, and achieve the effects of increasing dielectric constant, promoting polarity, and excellent mechanical properties
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[0018] The invention provides a method for preparing a high dielectric constant polymer-based dielectric composite material, comprising the following steps: uniformly mixing and dispersing an epoxy resin prepolymer, a curing agent, a catalyst, a solvent and an inorganic filler by a solution blending method, Forming an organic-inorganic composite slurry, the epoxy resin prepolymer has a polar group; coating the organic-inorganic composite slurry on a substrate; and heating and curing to obtain the high dielectric constant polymer base Dielectric composites.
[0019] In one embodiment of the present invention, the solution blending method is specifically as follows: First, based on the total weight of the organic-inorganic composite slurry to be formed, 25 to 35 wt% of epoxy resin prepolymer, 4 ~10wt% of curing agent and 0.15-0.3wt% of catalyst are added to 8~10wt% of the first solvent, and ultrasonically stirred at a temperature of 40~60°C for 30~40 minutes to obtain an organic...
Embodiment 1
[0034] The mark produced by Wuhan Ruifuyang Chemical Co., Ltd. is 21.3g of hydantoin epoxy resin MHR-018, the polyetheramine 18.5g of D2000 produced by U.S. Huntsman (Hunstman), DBU (diazabicyclo , also known as 1,8-diazabicycloundec-7-ene) curing agent 0.2g was added to 12.2g pentanone solvent, stirred and ultrasonicated at a temperature of 40°C for 30 minutes to obtain an organic prepolymer solution.
[0035] 55 g of inorganic filler barium titanate were dispersed in 16.5 g of pentanone solvent by ultrasonic stirring to obtain an inorganic suspension. The particle size of the inorganic filler barium titanate was nano-scale, purchased from Guangzhou Hongwu Material Technology Co., Ltd., particle size D 50 = between 0.1-1 μm.
[0036] Then the inorganic suspension is mixed with the above-mentioned organic prepolymer solution, and stirred uniformly by ultrasonic stirring to obtain a blended solution. The blended solution was poured into a ball mill jar and ball milled at a spe...
Embodiment 2
[0040] Add 25g of hydroxymethyl bisphenol A resin, 34.7g of phthalazinone, and 0.3g of cobalt acetylacetonate catalyst produced by Wuhan Yuancheng Gongchuang Nanjian Technology Co., Ltd. into 10g of methyl ethyl ketone solvent. Stir and sonicate for 30 minutes to obtain an organic prepolymer solution.
[0041] Ultrasonic stirring was used to disperse 60 g of the inorganic filler barium strontium titanate in 28 g of butyl acetate solvent to obtain an inorganic suspension. The inorganic filler barium strontium titanate is a nano-powder with a particle size of 20-500nm. Its preparation method is to first prepare a titanium-citric acid-ethylene glycol solution, and then add BaCO 3 , SrCO 3 Add the above solution to obtain a stable strontium barium titanate sol; then dry the strontium barium titanate sol at 80-120°C to form a xerogel; then heat treat at 600-800°C to obtain barium strontium titanate nanopowder .
[0042] Then the inorganic suspension is mixed with the above-menti...
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