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Photothermal conversion absorbing membrane system and sol-gel preparation method thereof

A light-to-heat conversion and absorption film technology, which is applied in chemical instruments and methods, heating devices, solar thermal devices, etc., can solve the problems of increasing the complexity of the film preparation process, the cost of film preparation, the high cost of film preparation, and the existence of danger , to achieve the effect of simple preparation method, low equipment requirements and low cost

Inactive Publication Date: 2012-10-31
FUZHOU UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

In 1997, Kraus et al reported the preparation of a sol with aluminum tri-sec-butoxide and nickel 2-ethylhexanoate [J. Appl. Phys., 821189-1195 (1997)], which was calcined at 1200°C to form NiAl2 O4, and then reduced with H2 at 950°C to prepare Ni-Al2O3Composite film, but this method requires high temperature and uses explosive H2, so the cost of film preparation is high, and it is also dangerous
In 2006, Westin et al. reported the method of preparing Al2O3-based thin films by solution chemistry. They prepared Al2 by using aluminum isopropoxide as raw material. O3 sol, but precipitation is inevitable during the process, and it takes a long time to stand and separate the clear liquid before it can be used for coating, which increases the complexity of the film preparation process and film preparation costs [Composite materials and method of its manufacture WO 2006 / 073357 A1]

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0027] best practice

[0028] 1. Take 50mL of absolute ethanol, add 4mL of acetylacetone and 11.6g of nickel nitrate hexahydrate in sequence under stirring, and stir for 1 hour to obtain a 0.8mol / L nickel sol.

[0029] 2. Take 20mL of 0.8mol / L nickel sol, and add 12mL of absolute ethanol under stirring to obtain a nickel sol with a concentration of 0.5mol / L.

[0030] 3. Add 8.2g of aluminum isopropoxide powder into 50mL of absolute ethanol, reflux with stirring and raise the temperature to 70°C, continue to stir and reflux for 1h, add 5mL of acetylacetone and 10.3mL of HCl, stir and reflux for 3h to obtain 0.8mol / L aluminum sol.

[0031] 4. Take 20mL of 0.8mol / L aluminum sol, and add 12mL of absolute ethanol under stirring to obtain an aluminum sol with a concentration of 0.5mol / L.

[0032]5. Add 10.4mL tetraethyl orthosilicate to 10mL absolute ethanol at room temperature and mix well, then continue to drop 3.6mL aqueous solution containing 0.06wt% HCl to it, and stir in a...

Embodiment 2

[0040] 1. Take 50mL of absolute ethanol, add 4mL of acetylacetone and 10.0g of cobalt acetate tetrahydrate in sequence under stirring, and stir for 1 hour to obtain 0.8mol / L cobalt sol.

[0041] 2. Take 20mL of 0.8mol / L cobalt sol, and add 12mL of absolute ethanol under stirring to obtain a cobalt sol with a concentration of 0.5mol / L.

[0042] 3. Add 8.2g of aluminum isopropoxide powder into 50mL of absolute ethanol, reflux with stirring and raise the temperature to 70°C, continue to stir and reflux for 1h, add 5mL of acetylacetone and 10.3mL of HCl, stir and reflux for 3h to obtain 0.8mol / L Aluminum sol.

[0043] 4. Take 20mL of 0.8mol / L aluminum sol, and add 12mL of absolute ethanol under stirring to obtain an aluminum sol with a concentration of 0.5mol / L.

[0044] 5. Add 10.4mL tetraethyl orthosilicate to 10mL absolute ethanol at room temperature and mix well, then continue to drop 3.6mL aqueous solution containing 0.06wt% HCl to it, and stir in a closed container for 24h ...

Embodiment 3

[0052] 1. Take 50mL of absolute ethanol, add 4mL of acetylacetone and 6.8g of copper chloride dihydrate in sequence under stirring, and stir for 1 hour to obtain 0.8mol / L copper sol.

[0053] 2. Take 20mL of 0.8mol / L copper sol, and add 12mL of absolute ethanol under stirring to obtain a copper sol with a concentration of 0.5mol / L.

[0054] 3. Add 8.2g of aluminum isopropoxide powder into 50mL of absolute ethanol, reflux with stirring and raise the temperature to 70°C, continue to stir and reflux for 1h, add 5mL of acetylacetone and 10.3mL of HCl, stir and reflux for 3h to obtain 0.8mol / L Aluminum sol.

[0055] 4. Take 20mL of 0.8mol / L aluminum sol, and add 12mL of absolute ethanol under stirring to obtain an aluminum sol with a concentration of 0.5mol / L. .

[0056] 5. Add 10.4mL tetraethyl orthosilicate to 10mL absolute ethanol at room temperature and mix well, then continue to drop 3.6mL aqueous solution containing 0.06wt% HCl to it, and stir in a closed container for 24h ...

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PUM

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Abstract

The invention provides a photothermal conversion absorbing membrane system and a sol-gel preparation method thereof, wherein the photothermal conversion membrane system is a three-layer structure consisting of two layers of alumina-based absorbing membranes with gradually changed ingredients on a metal substrate and an antireflective top layer; the two layers of alumina-based absorbing membranes with gradually changed ingredients adopt M-Al2O3 mixed sol with high metal content for the preparation of an absorbing bottom layer and adopts M-Al2O3 mixed sol with medium metal content for the preparation of an absorbing intermediate layer; the M represents the metal source in transition metal inorganic salts or transition metal organic salts; and the membrane system is prepared by sol-gel method. The photothermal conversion membrane system of the invention is low in cost and simple in preparation method, causes no environmental pollution and has high solar photothermal conversion efficiency.

Description

technical field [0001] The invention belongs to the technical field of functional materials, and relates to a photothermal conversion absorption film system and a sol-gel preparation method thereof. Background technique [0002] The solar light-to-heat conversion absorbing film is the most important and core part of the solar collector, and its optical properties affect the light-to-heat conversion efficiency of solar energy. M-Al 2 o 3 Composite thin film is a kind of cermet thin film, which has excellent solar energy absorption rate and high temperature thermal stability, and is widely used in solar collectors. At present, common thin film preparation methods include physical vapor deposition such as vacuum evaporation, sputtering coating and ion plating, and electrochemical deposition such as electroplating and anodic oxidation. Harmful substances such as phosphate and cyanide are used in the electrochemical method, which seriously pollutes the environment; although t...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B32B9/04F24J2/48B32B15/00C23C26/00
CPCY02E10/40
Inventor 赵剑曦李镇祥廖新焕姜蓉
Owner FUZHOU UNIV