This invention relates to the field of room-temperature
semiconductor radiation detector materials and device fabrication technology, and discloses a method for growing CsPbBr3 single crystals using a simple
solvent system. The invention employs a simple mixed
organic solvent system composed of
dimethyl sulfoxide (DMSO) and n-
butanol to grow CsPbBr3 single crystals using a reverse-temperature
crystallization method. This DMSO + n-
butanol solvent system can broaden the reverse-temperature range of CsPbBr3, enabling stable
crystal growth at lower temperatures and reducing the
crystal growth temperature. The n-
butanol additive can also regulate the
dissolution-coordination balance in the precursor solution, making the
crystal growth process smoother, reducing crystal defect density, and improving crystal quality. Furthermore, compared to
crystal growth using other complex
solvent systems, the simple DMSO + n-butanol
solvent system used in this invention has a clear composition and is easy to operate, which is beneficial for improving the stability and
repeatability of
crystal growth. The CsPbBr3 single crystals prepared by this method have good crystal quality and electrical properties, and can be applied in optoelectronic devices such as room-temperature
semiconductor radiation detectors.