The invention discloses a dual-layer-hybrid-array-based estimation method for a direction angle of arrival. With the method, problems of high operation load, a few of identification signal sources, and large estimation error in the prior art can be solved. The method comprises the following steps: (1), a one-layer coprime array and a two-layer nesting array are constructed respectively; (2), an output signal of the one-layer coprime array and an output signal of the two-layer nesting array are obtained; (3), on the basis of the output signal of the one-layer coprime array and the output signal of the two-layer nesting array, all four-order cumulants are calculated to form a four-order cumulant vector; (4), according to the four-order cumulant vector, an over-complete base is constructed and an airspace sparse vector is defined; (5), detection airspace direction-angle-of-arrival estimation is converted into sparse constraint equation solving; (6), with a convex optimization method, a sparest solution of an airspace sparse vector is obtained; and (7), an amplitude spectrogram is drawn based on the sparest solution and a direction angle of arrival is obtained. According to the method provided in the invention, the signal source number with identifiable arrays increases substantially under the circumstance that the array element number is limited. The method is suitable for target scouting and passive location.