The invention discloses a tooth glaze composition, a tooth glaze forming method and a denture prosthesis. The tooth glaze composition comprises, by mass, 53-65% of SiO2, 6-15% of B2O3, 8-12% of Na2O, 6-8% of K2O, 1-3% of Li2O, 2-5% of an alkaline earth metal oxide, 5.5-11% of Al2O3 and 0.5-2% of ZrO2, and the alkaline earth metal oxide is CaO or a mixture of CaO and SrO. The tooth glaze composition disclosed by the invention has a relatively low sintering temperature, and the application range of the tooth glaze composition is widened, so that the tooth glaze composition not only can be applied to restoration matrixes of zirconium oxide, metal and the like with high melting temperature, but also can be applied to restoration matrixes of glass ceramics, cast porcelain, baked porcelain and the like with low melting temperature.