The invention relates to the field of rubber and particularly relates to a tire air-tight layer rubber composite containing a nano filler StronWiNTC. The tire air-tight layer rubber composite is characterized by comprising the following raw materials in parts by weight: 25-45 parts of natural rubber, 20-40 parts of butylbenzene rubber, 15-55 parts of chlorinated butyl rubber, 52-60 parts of carbon black N660, 20-28 parts of StronWiNTC, 4-6 parts of aromatic hydrocarbon oil, 3-5 parts of zinc oxide, 1-2 parts of stearic acid, 1-2 parts of anti-ageing agent 4020, 1-2 parts of anti-ageing agent RD, 3-4 parts of protective wax OK5194, 3-4 parts of tackifying resin A-90, 1-2 parts of accelerator TMTD (Tetramethylthiuram Disulfide), 1-2 parts of accelerator CZ and 0.5-1.0 part of vulcanizing agent WP5. The tire air-tight layer rubber composite disclosed by the invention can endow good mechanical property and heat stability to the air-tight layer and can improve the air tightness of air-tight layer rubber; and particularly, the tire air-tight layer rubber composite has appropriate advantages on the aspects of performances of elasticity, flexing resistance, stable size, separation performance, elongation at rupture, compression and deformation and the like.