The invention provides relates to connection technologies for carbon nanometer tube macroscopic films or fibers and metal in the technical field of nanometer materials, in particular to a method for connecting a carbon nanometer tube macroscopic material with metal. The method sequentially comprises the following steps that the portion, needing to be connected, of line-shaped or band-shaped metallic copper or metallic aluminum or metallic tin is ground, polished, washed with ethyl alcohol and dried; carbon nanometer tube macroscopic films or fibers are well prepared, 0.01 mL to 10 mL of elargol is cured at a room temperature, after it is guaranteed that the condition that the curing electric resistivity is kept between 0.002 Ohm / cm to 0.01 Ohm / cm is met, the portion, needing to be connected, of the carbon nanometer tube macroscopic material is coated with the elargol through a needle point of an injector, the metallic portion needing to be connected with the carbon nanometer tube macroscopic material is placed on the surface coated with the elargol, the metal is tightly pressed through a steel ruler, and then the metal can be completely connected with the carbon nanometer tube macroscopic films or fibers. By the adoption of the method for connecting the carbon nanometer tube macroscopic material with the metal, the obtained contact resistance between carbon nanometer tube macroscopic material and the metal is reduced to within 10 Ohms, the technology is simple, and cost is low.