The invention provides a method of using satellite rolling-axis rapid attitude manoeuvre to unload the angular momentum of a rolling axis and a yawing axis, and belongs to the technical field of spacecraft attitude control. The method resolves the problems that at present, an unloading device needs to be additionally installed on a satellite to unload the angular momentum absorbed by momentum exchange actuating mechanisms of the satellite, and therefore manufacturing cost of the satellite is increased, and the size and the weight of the satellite are increased. A body system and an inertial coordinate system of the satellite are defined, and an initial unloading moment is confirmed; and unloading is conducted by means of confirmation of the gravity gradient force moment borne by the satellite, accumulated angular momentum vectors of the gravity gradient force moment inside each orbital period, the angular momentum, needing to be unloaded, of all the momentum exchange actuating mechanisms on the rolling axis, the angular momentum, needing to be unloaded, of all the momentum exchange actuating mechanisms on the yawing axis, the number of turns of unloaded orbits of the satellite, the maneuvering angle in a satellite unloading process, and time used by the satellite rolling-axis maneuvering angle. The method can be widely applied to accumulated angular momentum unloading requirements of the actuating mechanisms.