Disclosed are a device and method for trapping carbon resources in the atmosphere. The method includes the following steps: (1), transferring gaseous CO2 in the atmosphere into the biosphere to form solid organic carbon compounds through photosynthesis of rank vegetation, trapping CO2 in the atmosphere, and converting the CO2 into organic carbon compounds through microorganisms or enzyme, (2), trapping CO2 in the atmosphere in a physical method, (3), trapping CO2 in the atmosphere in a chemical method, (4), trapping CO2 in the atmosphere in a physicochemical method, and (5), carrying out carbon storage and sealing storage on the carbon resources trapped from the atmosphere to achieve negative growth of atmospheric CO2, reduce partial pressure of atmospheric CO2 gas, adjust the greenhouse effect and solve relevant environmental problems, putting the stored carbon products into global carbon trading, and carrying out technical control over the cyclic process of carbon cycle, carbon conversion, carbon storage, carbon sealing storage and carbon utilization so that people can use carbon sources fully and reasonably. Manual cultivation and planting of the rank vegetation are new power for carbon cycles on the earth.